Recent advances and future perspectives of metal-organic frameworks as efficient electrocatalysts for CO2 reduction

IF 6.8 2区 材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Science China Materials Pub Date : 2024-11-08 DOI:10.1007/s40843-024-3165-6
Chao Li  (, ), Hong Yan  (, ), Hanlu Yang  (, ), Wenqian Zhou  (, ), Chengyu Xie  (, ), Baocai Pan  (, ), Qichun Zhang  (, )
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Abstract

The conversion of carbon dioxide (CO2) to the reduced chemical compounds offers substantial environmental benefits through minimizing the emission of greenhouse gas and fostering sustainable practices. Recently, the unique properties of metal-organic frameworks (MOFs) make them attractive candidates for electrocatalytic CO2 reduction reaction (CO2RR), providing many opportunities to develop efficient, selective, and environmentally sustainable processes for mitigating CO2 emissions and utilizing CO2 as a valuable raw material for the synthesis of fuels and chemicals. Here, the recent advances in MOFs as efficient catalysts for electrocatalytic CO2RR are summarized. The detailed characteristics, electrocatalytic mechanisms, and practical approaches for improving the electrocatalytic efficiency, selectivity, and durability of MOFs under realistic reaction conditions are also clarified. Furthermore, the outlooks on the prospects of MOF-based electrocatalysts in CO2RR are provided.

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金属-有机骨架作为高效二氧化碳还原电催化剂的研究进展与展望
将二氧化碳(CO2)转化为减少的化合物,通过最大限度地减少温室气体的排放和促进可持续的做法,提供了巨大的环境效益。最近,金属有机框架(mof)的独特性质使其成为电催化二氧化碳还原反应(CO2RR)的有吸引力的候选者,为开发高效、选择性和环境可持续的工艺提供了许多机会,以减少二氧化碳排放,并利用二氧化碳作为合成燃料和化学品的宝贵原料。本文综述了mof作为电催化CO2RR高效催化剂的研究进展。阐明了mof的详细特性、电催化机理以及在实际反应条件下提高电催化效率、选择性和耐久性的可行方法。展望了mof基CO2RR电催化剂的发展前景。
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来源期刊
Science China Materials
Science China Materials Materials Science-General Materials Science
CiteScore
11.40
自引率
7.40%
发文量
949
期刊介绍: Science China Materials (SCM) is a globally peer-reviewed journal that covers all facets of materials science. It is supervised by the Chinese Academy of Sciences and co-sponsored by the Chinese Academy of Sciences and the National Natural Science Foundation of China. The journal is jointly published monthly in both printed and electronic forms by Science China Press and Springer. The aim of SCM is to encourage communication of high-quality, innovative research results at the cutting-edge interface of materials science with chemistry, physics, biology, and engineering. It focuses on breakthroughs from around the world and aims to become a world-leading academic journal for materials science.
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