{"title":"In-situ gamma-ray measurement to estimate depth distribution of 137Cs in farmland in Fukushima Prefecture","authors":"Sadao Momota , Yoshihiro Okuda , Minoru Tanigaki , Yoshitaka Ohkubo , Takashi Saito","doi":"10.1016/j.jenvrad.2024.107610","DOIUrl":null,"url":null,"abstract":"<div><div>Radioactive cesium released into the atmosphere caused by the Fukushima Dai-ichi Nuclear Power Plant accident in March 2011 has contaminated the surrounding area. We confirmed the applicability of in-situ methods to evaluate the depth distribution of <sup>137</sup>Cs by employing the ratio of Compton-scattering and photo-peak components (<em>r</em><sub>C</sub>) obtained from measured gamma-ray spectra. In the present study, we applied the in-situ method to farmlands in Fukushima Prefecture whose sites were disturbed by decontamination and plowing operations. <em>r</em><sub>C</sub> and the net count of the 662-keV photo-peak, <em>n</em><sub>peak</sub>, were obtained from gamma-ray spectra measured using a portable CsI detector. Reasonable <em>r</em><sub>C</sub> was obtained by removing the contribution of naturally occurring radioactive materials through a simple and versatile procedure. The depth distribution of <sup>137</sup>Cs measured using the conventional sampling method was reproduced using the Fermi distribution function. The concentration of <sup>137</sup>Cs on the ground surface, <em>N</em>(0), and the depth at which the concentration becomes half of <em>N</em>(0), <em>d</em><sub>1/2</sub>, can be described by simple functions of <em>n</em><sub>peak</sub> and <em>r</em><sub>C</sub>, respectively. We also confirmed that the Monte Carlo simulation is useful to reproduce the present results, taking into account the contribution of <sup>134</sup>Cs and the detection system properly.</div></div>","PeriodicalId":15667,"journal":{"name":"Journal of environmental radioactivity","volume":"282 ","pages":"Article 107610"},"PeriodicalIF":1.9000,"publicationDate":"2025-02-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Journal of environmental radioactivity","FirstCategoryId":"93","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S0265931X2400242X","RegionNum":3,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"ENVIRONMENTAL SCIENCES","Score":null,"Total":0}
引用次数: 0
Abstract
Radioactive cesium released into the atmosphere caused by the Fukushima Dai-ichi Nuclear Power Plant accident in March 2011 has contaminated the surrounding area. We confirmed the applicability of in-situ methods to evaluate the depth distribution of 137Cs by employing the ratio of Compton-scattering and photo-peak components (rC) obtained from measured gamma-ray spectra. In the present study, we applied the in-situ method to farmlands in Fukushima Prefecture whose sites were disturbed by decontamination and plowing operations. rC and the net count of the 662-keV photo-peak, npeak, were obtained from gamma-ray spectra measured using a portable CsI detector. Reasonable rC was obtained by removing the contribution of naturally occurring radioactive materials through a simple and versatile procedure. The depth distribution of 137Cs measured using the conventional sampling method was reproduced using the Fermi distribution function. The concentration of 137Cs on the ground surface, N(0), and the depth at which the concentration becomes half of N(0), d1/2, can be described by simple functions of npeak and rC, respectively. We also confirmed that the Monte Carlo simulation is useful to reproduce the present results, taking into account the contribution of 134Cs and the detection system properly.
期刊介绍:
The Journal of Environmental Radioactivity provides a coherent international forum for publication of original research or review papers on any aspect of the occurrence of radioactivity in natural systems.
Relevant subject areas range from applications of environmental radionuclides as mechanistic or timescale tracers of natural processes to assessments of the radioecological or radiological effects of ambient radioactivity. Papers deal with naturally occurring nuclides or with those created and released by man through nuclear weapons manufacture and testing, energy production, fuel-cycle technology, etc. Reports on radioactivity in the oceans, sediments, rivers, lakes, groundwaters, soils, atmosphere and all divisions of the biosphere are welcomed, but these should not simply be of a monitoring nature unless the data are particularly innovative.