A linearly polarized AC-driven perovskite light emitting device with nanoscale metal contact†

IF 5.1 3区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY Nanoscale Pub Date : 2025-01-15 DOI:10.1039/D4NR04894F
Li-Ming Chiang, Chi-Peng Tu, James Singh Konthoujam, Hai-Pang Chiang, Tsung-Sheng Kao and Min-Hsiung Shih
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Abstract

Electroluminescent (EL) devices consisting of a single metal–semiconductor contact and a gate effect structure have garnered significant attention in the field of perovskite light-emitting devices. This interest is largely due to the thermal stability of the active layer and the simplicity of the device structure. However, the application of these devices in large-area light-emitting applications is hindered by the inherently low carrier mobility in perovskite materials. In our study, we addressed this limitation by optimizing the nanostructure within the electrodes, which resulted in enhanced electroluminescence and linear polarization. To confirm the luminescence mechanism and the observed enhancement, we conducted comprehensive electrical and optical characterization studies. These characterization studies demonstrated the effectiveness of our approach in improving the performance of perovskite-based EL devices, paving the way for their broader application in large-area light-emitting technologies.

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纳米级金属触点线极化交流驱动钙钛矿发光器件
在钙钛矿发光器件领域,由单一金属-半导体触点和门效应结构组成的电致发光器件受到了广泛的关注。这种兴趣主要是由于有源层的热稳定性和器件结构的简单性。然而,钙钛矿材料固有的低载流子迁移率阻碍了这些器件在大面积发光应用中的应用。在我们的研究中,我们通过优化电极内的纳米结构来解决这一限制,从而增强了电致发光和线极化。为了确认发光机制和观察到的增强,我们进行了全面的电学和光学表征。这些表征证明了我们的方法在提高钙钛矿基EL器件性能方面的有效性,为其在大面积发光技术中的更广泛应用铺平了道路。
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来源期刊
Nanoscale
Nanoscale CHEMISTRY, MULTIDISCIPLINARY-NANOSCIENCE & NANOTECHNOLOGY
CiteScore
12.10
自引率
3.00%
发文量
1628
审稿时长
1.6 months
期刊介绍: Nanoscale is a high-impact international journal, publishing high-quality research across nanoscience and nanotechnology. Nanoscale publishes a full mix of research articles on experimental and theoretical work, including reviews, communications, and full papers.Highly interdisciplinary, this journal appeals to scientists, researchers and professionals interested in nanoscience and nanotechnology, quantum materials and quantum technology, including the areas of physics, chemistry, biology, medicine, materials, energy/environment, information technology, detection science, healthcare and drug discovery, and electronics.
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