Composite solid-state electrolytes for all solid-state lithium batteries: progress, challenges and outlook

IF 3.2 Q2 CHEMISTRY, PHYSICAL Energy advances Pub Date : 2024-12-17 DOI:10.1039/D4YA00542B
Senhao Wang, Andrea La Monaca and George P. Demopoulos
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Abstract

Composite solid-state electrolytes (CSEs) with multiple phases offer greater flexibility to customize and combine the advantages of single-phase electrolytes, making them promising candidates for commercial all-solid-state batteries (ASSBs). Based on existing investigations, this review provides a comprehensive overview of the recent progress in CSEs. First, we introduce the historical development of solid-state ionic conductors, and then summarize the fundamentals including key materials and mechanisms of lithium-ion transport. Three main types of advanced structures for CSEs are classified and highlighted according to the recent progress, namely composite solid electrolytes with passive fillers, composite solid electrolytes with active fillers, and 3D framework composite solid electrolytes. Finally, the challenges and perspectives of the composite solid-state electrolytes are discussed.

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用于所有固态锂电池的复合固态电解质:进展、挑战和展望
多相复合固态电解质(cse)提供了更大的灵活性,可以定制和结合单相电解质的优点,使其成为商用全固态电池(assb)的有希望的候选者。本文在现有研究的基础上,对近年来的研究进展进行了综述。本文首先介绍了固态离子导体的发展历史,然后总结了锂离子输运的基本原理,包括关键材料和输运机理。根据近年来的研究进展,将cse先进结构分为三种主要类型,即无源填料复合固体电解质、有源填料复合固体电解质和三维框架复合固体电解质。最后,讨论了复合固态电解质面临的挑战和发展前景。
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