Quantitative analysis of particle behavior constituting multiple coherent structures in liquid bridges

IF 9.4 1区 化学 Q1 CHEMISTRY, PHYSICAL Journal of Colloid and Interface Science Pub Date : 2025-01-09 DOI:10.1016/j.jcis.2024.12.168
Shin Noguchi , Ichiro Ueno
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Abstract

Hypothesis

Coherent structures by low-Stokes-number particles are induced within a closed flow, in which ordered flow regions known as Kolmogorov-Arnold-Moser (KAM) tori emerge. A variety of structures with different spatial characteristics has been predicted by varying the Stokes number, whereas the coexistence of structures in flow suspending various types of particles has not been hitherto demonstrated.

Experiments

Half-zone liquid bridges of O (
) are prepared as a closed system to induce thermocapillary-driven time-dependent flow under normal gravity conditions. By suspending single or multiple types of particles of O (
) in diameter, we track the particle trajectories with two synchronized high-speed cameras and count the particles forming coherent structures.

Findings

The coexistence of various coherent structures is unveiled in systems where particle groups of different diameters are simultaneously suspended. We demonstrate the constitution of multiple coherent structures in the reference frame rotating with traveling wave: Some structures are dominated by a single type of particles, whereas some others are composed by various type of particles. Through a quantitative evaluation of the number of particles forming each manifested coherent structure, “the attractivity” of structures is discussed.

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液体桥中构成多重相干结构的粒子行为的定量分析。
假设:低斯托克斯数粒子在封闭流动中诱导出相干结构,其中出现了称为Kolmogorov-Arnold-Moser (KAM)环面的有序流动区域。通过改变斯托克斯数可以预测出具有不同空间特征的多种结构,而悬浮在不同类型颗粒中的流动结构的共存迄今尚未得到证实。实验:制备O()半区液桥作为封闭体系,在正常重力条件下诱导热毛细管驱动的时间相关流动。通过悬挂直径为0()的单一或多种类型的粒子,用两台同步高速摄像机跟踪粒子轨迹,并对形成相干结构的粒子进行计数。发现:在不同直径的粒子群同时悬浮的体系中,揭示了多种相干结构的共存。我们论证了行波旋转参照系中多重相干结构的构成:一些结构由单一类型的粒子主导,而另一些结构由多种类型的粒子组成。通过对形成每一相干结构的粒子数量的定量评价,讨论了结构的“吸引力”。
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来源期刊
CiteScore
16.10
自引率
7.10%
发文量
2568
审稿时长
2 months
期刊介绍: The Journal of Colloid and Interface Science publishes original research findings on the fundamental principles of colloid and interface science, as well as innovative applications in various fields. The criteria for publication include impact, quality, novelty, and originality. Emphasis: The journal emphasizes fundamental scientific innovation within the following categories: A.Colloidal Materials and Nanomaterials B.Soft Colloidal and Self-Assembly Systems C.Adsorption, Catalysis, and Electrochemistry D.Interfacial Processes, Capillarity, and Wetting E.Biomaterials and Nanomedicine F.Energy Conversion and Storage, and Environmental Technologies
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