Single-crystal CsPbBr3-based vertical cavity surface emitting laser.

IF 3.1 2区 物理与天体物理 Q2 OPTICS Optics letters Pub Date : 2025-01-15 DOI:10.1364/OL.547212
Shunya Aoyagi, Zhan Su, Gouen Weng, Shoujie Ye, Fuyi Cao, Cong Wang, Xiaobo Hu, Yohei Yamamoto, Shaoqiang Chen
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Abstract

All-inorganic perovskite materials have been widely used in various devices, including lasers, light-emitting diodes (LEDs), and solar cells, due to their exceptional optoelectronic properties. Devices utilizing high-quality single crystals are anticipated to achieve significantly enhanced performance. In this work, we present a high-performance vertical cavity surface emitting laser (VCSEL) based on a single-crystal CsPbBr3 microplatelet, fabricated through a simple solution process and sandwiched between two distributed Bragg reflector (DBRs). The VCSEL demonstrated single-mode lasing at 542 nm, a low threshold of 5 µJ/cm2, and a high Q-factor of 2893. Additionally, time-resolved photoluminescence (TRPL) measurements using a streak camera revealed picosecond-scale lasing dynamics. This study offers a novel, to the best of our knowledge, approach for realizing laser devices using perovskite single-crystal microplatelets.

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单晶cspbbr3基垂直腔面发射激光器。
由于其优异的光电性能,全无机钙钛矿材料已广泛应用于各种器件,包括激光器,发光二极管(led)和太阳能电池。利用高质量单晶的器件有望实现显著增强的性能。在这项工作中,我们提出了一种高性能的垂直腔面发射激光器(VCSEL),该激光器基于单晶CsPbBr3微血小板,通过简单的溶液工艺制成,夹在两个分布式布拉格反射器(dbr)之间。VCSEL在542 nm处显示单模激光,低阈值为5µJ/cm2,高q因子为2893。此外,使用条纹相机进行的时间分辨光致发光(TRPL)测量显示了皮秒级的激光动力学。据我们所知,这项研究为使用钙钛矿单晶微血小板实现激光器件提供了一种新颖的方法。
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来源期刊
Optics letters
Optics letters 物理-光学
CiteScore
6.60
自引率
8.30%
发文量
2275
审稿时长
1.7 months
期刊介绍: The Optical Society (OSA) publishes high-quality, peer-reviewed articles in its portfolio of journals, which serve the full breadth of the optics and photonics community. Optics Letters offers rapid dissemination of new results in all areas of optics with short, original, peer-reviewed communications. Optics Letters covers the latest research in optical science, including optical measurements, optical components and devices, atmospheric optics, biomedical optics, Fourier optics, integrated optics, optical processing, optoelectronics, lasers, nonlinear optics, optical storage and holography, optical coherence, polarization, quantum electronics, ultrafast optical phenomena, photonic crystals, and fiber optics. Criteria used in determining acceptability of contributions include newsworthiness to a substantial part of the optics community and the effect of rapid publication on the research of others. This journal, published twice each month, is where readers look for the latest discoveries in optics.
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