Weak Antilocalization and Negative Magnetoresistance of the Gate-Tunable PbTe Thin Films

IF 4.6 2区 化学 Q2 CHEMISTRY, PHYSICAL The Journal of Physical Chemistry Letters Pub Date : 2025-01-27 DOI:10.1021/acs.jpclett.4c03425
Huizhen Li, Kang Li, Wenyu Hu, Jianyuan Zhao, Tong Su, Jielin Yang, Yiming Chen, Kuo Yang, Mei Du, Zhe Li, Weiwei Zhao
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Abstract

We have systematically studied the electromagnetic transport properties of PbTe thin films under gate voltage modulation. The system demonstrates pronounced electron–electron interactions exclusively within the gate voltage range where only hole carriers are present. Furthermore, the Berry phase is utilized to qualitatively elucidate the transition between weak antilocalization (WAL) and weak localization (WL) through the regulation of gate voltage and temperature. Using the three-resistor model, we have effectively explained the correlation between the characteristic temperature of the RT curve, the coexistence of electron–hole carriers, and the nonmonotonic temperature dependence of negative magnetoresistance (NMR), consistently indicating that complex magnetotransport phenomena are caused by microscopic disorder. Our research findings open up new avenues for exploring and manipulating the magnetotransport properties of PbTe thin films.

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栅极可调谐PbTe薄膜的弱反局域化和负磁阻
系统地研究了栅极电压调制下PbTe薄膜的电磁输运特性。在只有空穴载流子存在的栅电压范围内,系统显示出明显的电子-电子相互作用。此外,利用Berry相位定性地解释了通过栅极电压和温度的调节从弱反局域化(WAL)到弱局域化(WL)的转变。利用三电阻模型,我们有效地解释了R-T曲线的特征温度、电子-空穴载流子的共存以及负磁阻(NMR)的非单调温度依赖性之间的关系,一致地表明复杂磁输运现象是由微观无序引起的。我们的研究结果为探索和操纵PbTe薄膜的磁输运特性开辟了新的途径。
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来源期刊
The Journal of Physical Chemistry Letters
The Journal of Physical Chemistry Letters CHEMISTRY, PHYSICAL-NANOSCIENCE & NANOTECHNOLOGY
CiteScore
9.60
自引率
7.00%
发文量
1519
审稿时长
1.6 months
期刊介绍: The Journal of Physical Chemistry (JPC) Letters is devoted to reporting new and original experimental and theoretical basic research of interest to physical chemists, biophysical chemists, chemical physicists, physicists, material scientists, and engineers. An important criterion for acceptance is that the paper reports a significant scientific advance and/or physical insight such that rapid publication is essential. Two issues of JPC Letters are published each month.
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