Identification and Screening of Trace and Multityped Solvents Using Transpiration-Driven Electrokinetic Generation Principle.

IF 9.1 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY Nano Letters Pub Date : 2025-02-12 Epub Date: 2025-01-30 DOI:10.1021/acs.nanolett.4c05840
Wenli Gao, Mengfei Yu, Leitao Cao, Piao Wen, Yi Sun, Jing Ren, Shengjie Ling
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Abstract

Transpiration-driven electrokinetic power generators (TEPGs) hold promising potential for intelligent chemical sensing applications, enabling the efficient identification and screening of organic solvents. Here, we report a novel TEPG-based chemical sensor using MoS2-doped cellulose filter paper for efficient detection of poplar solvents like water, alcohols, and methanol. TEPGs operate by leveraging capillary-driven transpiration to induce solvent flow through porous materials, leading to ion migration and the formation of electrical double layers (EDLs) at the solid-liquid interfaces. This process generates a potential difference, enabling the conversion of the mechanical transpiration energy into electrical signals. Integrated with machine learning algorithms and IoT technologies, the sensor achieves real-time classification of the solvents. This TEPG-CS system offers enhanced sensitivity, reliability, and operational adaptability, overcoming the limitations of the traditional detection methods. This work has broad potential for environmental monitoring, industrial applications, and biomedical fields, offering another pathway for advanced solvent detection and classification systems.

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利用蒸腾驱动的电动力产生原理鉴定和筛选痕量和多类型溶剂。
蒸腾驱动的电动发电机(tepg)在智能化学传感应用中具有广阔的潜力,可以有效地识别和筛选有机溶剂。在这里,我们报道了一种新型的基于tepg的化学传感器,该传感器使用二硫化钼掺杂纤维素滤纸,用于有效检测杨树溶剂,如水,醇和甲醇。tepg的工作原理是利用毛细管驱动的蒸腾作用诱导溶剂流过多孔材料,导致离子迁移,并在固液界面形成双电层(edl)。这个过程产生一个电位差,使机械蒸腾能转化为电信号。该传感器与机器学习算法和物联网技术相结合,实现了溶剂的实时分类。该TEPG-CS系统具有更高的灵敏度、可靠性和操作适应性,克服了传统检测方法的局限性。这项工作在环境监测、工业应用和生物医学领域具有广泛的潜力,为先进的溶剂检测和分类系统提供了另一条途径。
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来源期刊
Nano Letters
Nano Letters 工程技术-材料科学:综合
CiteScore
16.80
自引率
2.80%
发文量
1182
审稿时长
1.4 months
期刊介绍: Nano Letters serves as a dynamic platform for promptly disseminating original results in fundamental, applied, and emerging research across all facets of nanoscience and nanotechnology. A pivotal criterion for inclusion within Nano Letters is the convergence of at least two different areas or disciplines, ensuring a rich interdisciplinary scope. The journal is dedicated to fostering exploration in diverse areas, including: - Experimental and theoretical findings on physical, chemical, and biological phenomena at the nanoscale - Synthesis, characterization, and processing of organic, inorganic, polymer, and hybrid nanomaterials through physical, chemical, and biological methodologies - Modeling and simulation of synthetic, assembly, and interaction processes - Realization of integrated nanostructures and nano-engineered devices exhibiting advanced performance - Applications of nanoscale materials in living and environmental systems Nano Letters is committed to advancing and showcasing groundbreaking research that intersects various domains, fostering innovation and collaboration in the ever-evolving field of nanoscience and nanotechnology.
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