Promoting Yb₂Si₂O₇ environmental barrier coatings for service at 1425 °C

IF 6.2 2区 材料科学 Q1 MATERIALS SCIENCE, CERAMICS Journal of The European Ceramic Society Pub Date : 2025-01-09 DOI:10.1016/j.jeurceramsoc.2025.117200
Lin Chen , Shu-Wen Li , Chang-Jiu Li, Guan-Jun Yang
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Abstract

Si-based environmental barrier coatings (EBCs) are indispensable for SiC composites. However, the service temperature of next-generation composites exceeds 1400 °C, leading to melting of the Si bond coat. To mitigate this issue, Yb2Si2O7 (YbDS) and mullite/YbDS coatings without Si bond coat were proposed. The results indicate that YbDS coatings can survive for 150 h at 1425 °C, while mullite/YbDS coatings experienced significant spallation during this period. Both SiO2 phase transition and interfacial holes cause spallation of the YbDS and mullite/YbDS coatings. This research provides valuable insights for designing next-generation EBCs.
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推广Yb₂Si₂O₇环境屏障涂料,适用于1425°C
硅基环境屏障涂层是碳化硅复合材料不可缺少的材料。然而,下一代复合材料的使用温度超过1400℃,导致Si结合层熔化。为了解决这一问题,提出了不含硅结合层的Yb2Si2O7 (YbDS)和莫来石/YbDS涂层。结果表明,YbDS涂层在1425℃下可存活150 h,而莫来石/YbDS涂层在此期间发生了明显的剥落。SiO2相变和界面孔洞都是导致YbDS和莫来石/YbDS涂层剥落的原因。本研究为下一代EBCs的设计提供了有价值的见解。
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来源期刊
Journal of The European Ceramic Society
Journal of The European Ceramic Society 工程技术-材料科学:硅酸盐
CiteScore
10.70
自引率
12.30%
发文量
863
审稿时长
35 days
期刊介绍: The Journal of the European Ceramic Society publishes the results of original research and reviews relating to ceramic materials. Papers of either an experimental or theoretical character will be welcomed on a fully international basis. The emphasis is on novel generic science concerning the relationships between processing, microstructure and properties of polycrystalline ceramics consolidated at high temperature. Papers may relate to any of the conventional categories of ceramic: structural, functional, traditional or composite. The central objective is to sustain a high standard of research quality by means of appropriate reviewing procedures.
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