Sodium Alginate Composite Films Incorporated by Glycerol and Oxidized MWCNT for Driving Dielectric Elastomers

IF 3.6 3区 化学 Q2 POLYMER SCIENCE Journal of Polymer Science Pub Date : 2024-12-05 DOI:10.1002/pol.20240734
Chuang Li, Chenyu Xu, Xiangyu Song, Li Ma, Dehai Zhang, Dongjie Guo
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Abstract

Dielectric elastomer actuators (DEAs) are widely used in many fields such as bionic robotics and wearable electronics. Due to a high elastic modulus and a poor flexibility, pure sodium alginate (SA) film constrains the deflection of DEA and is not suitable for using as the electrode. By incorporating the plasticizer of glycerol and the conductive fillers of oxidized multi-walled carbon nanotubes (MWCNTs), the resultant MWCNT/SA composite film exhibits a high flexibility and a high electrical conductivity (129 Ω·sq.−1), enabling it as the electrode to drive the dielectric matrix of VHB4910 for out-of-plane actuations. Driven by a relatively low electric field of 20.8 V/μm, the MWCNT/SA electrode DEA presents a desired areal strain of 3.8%. Long-term actuations reveal that the MWCNT/SA electrode DEA exhibits very stable electromechanical behaviors with a relative displacement shift (RDS) of 19.8% over 500 cycles, which is far lower than the commercial silicone electrode DEA, whose RDS is 127.8% under the same driven conditions.

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甘油-氧化MWCNT海藻酸钠复合膜驱动介电弹性体
介电弹性体致动器广泛应用于仿生机器人、可穿戴电子等领域。纯海藻酸钠(SA)膜弹性模量高,柔韧性差,限制了DEA的偏转,不适合作为电极使用。通过加入增塑剂甘油和氧化多壁碳纳米管(MWCNTs)的导电填料,得到的MWCNT/SA复合膜具有高柔韧性和高导电性(129 Ω·sq.−1),使其能够作为电极驱动VHB4910的介电矩阵进行面外驱动。在相对较低的20.8 V/μm电场驱动下,MWCNT/SA电极DEA的期望面应变为3.8%。长期驱动表明,MWCNT/SA电极DEA表现出非常稳定的机电行为,在500次循环中相对位移位移(RDS)为19.8%,远低于商业硅胶电极DEA在相同驱动条件下的RDS为127.8%。
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来源期刊
Journal of Polymer Science
Journal of Polymer Science POLYMER SCIENCE-
CiteScore
6.30
自引率
5.90%
发文量
264
期刊介绍: Journal of Polymer Research provides a forum for the prompt publication of articles concerning the fundamental and applied research of polymers. Its great feature lies in the diversity of content which it encompasses, drawing together results from all aspects of polymer science and technology. As polymer research is rapidly growing around the globe, the aim of this journal is to establish itself as a significant information tool not only for the international polymer researchers in academia but also for those working in industry. The scope of the journal covers a wide range of the highly interdisciplinary field of polymer science and technology.
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