Ferromagnetic-like magnetic interactions in Ge1-x-ySixMnyTe multiferroics

IF 2.4 4区物理与天体物理 Q3 PHYSICS, CONDENSED MATTER Solid State Communications Pub Date : 2025-03-01 Epub Date: 2024-12-27 DOI:10.1016/j.ssc.2024.115812

Sana Zakar , Abdul Khaliq , Mujeeb Ahmad , Vasyl E. Slynko , Lukasz Kilanski

{"title":"Ferromagnetic-like magnetic interactions in Ge1-x-ySixMnyTe multiferroics","authors":"Sana Zakar , Abdul Khaliq , Mujeeb Ahmad , Vasyl E. Slynko , Lukasz Kilanski","doi":"10.1016/j.ssc.2024.115812","DOIUrl":null,"url":null,"abstract":"<div><div>IV-VI materials doping with magnetic impurities presents exciting opportunities for spintronic applications particularly by incorporating the memory component in the semiconducting matrix. The proposed work investigates carrier mediated magnetic interactions in GeTe lattice alloyed with Mn ions. We present Ge<sub>1-x-y</sub>Si<sub>x</sub>Mn<sub>y</sub>Te bulk crystals having a chemical composition of Si, <em>x</em> = 0.057, 0.053 and Mn, <em>y</em> = 0.035, 0.041 to explore the dominant magnetic interactions in these crystals. The results show that magnetic phase transition temperature for both crystals is closer to 170 K, with the Curie-Weiss temperature (<span><math><mrow><mi>θ</mi></mrow></math></span>) calculated as 171 K for <em>y</em> = 0.035 and 172.8 K for <em>y</em> = 0.041, indicating ferromagnetic-like interactions amongst Mn ions. An increase in Mn content from <em>y</em> = 0.035 to 0.041, the maxima of susceptibility cusp amplify about an order of magnitude. Modified Curie-Weiss law fits on susceptibility inverse finds ferromagnetic-like interaction in the alloys. Additionally, high field magnetization data was used for calculating the number of active magnetic ions in semiconductor matrix.</div></div>","PeriodicalId":430,"journal":{"name":"Solid State Communications","volume":"397 ","pages":"Article 115812"},"PeriodicalIF":2.4000,"publicationDate":"2025-03-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Solid State Communications","FirstCategoryId":"101","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S0038109824003892","RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"2024/12/27 0:00:00","PubModel":"Epub","JCR":"Q3","JCRName":"PHYSICS, CONDENSED MATTER","Score":null,"Total":0}

引用次数: 0

Abstract

IV-VI materials doping with magnetic impurities presents exciting opportunities for spintronic applications particularly by incorporating the memory component in the semiconducting matrix. The proposed work investigates carrier mediated magnetic interactions in GeTe lattice alloyed with Mn ions. We present Ge_1-x-ySi_xMn_yTe bulk crystals having a chemical composition of Si, x = 0.057, 0.053 and Mn, y = 0.035, 0.041 to explore the dominant magnetic interactions in these crystals. The results show that magnetic phase transition temperature for both crystals is closer to 170 K, with the Curie-Weiss temperature (

θ

) calculated as 171 K for y = 0.035 and 172.8 K for y = 0.041, indicating ferromagnetic-like interactions amongst Mn ions. An increase in Mn content from y = 0.035 to 0.041, the maxima of susceptibility cusp amplify about an order of magnitude. Modified Curie-Weiss law fits on susceptibility inverse finds ferromagnetic-like interaction in the alloys. Additionally, high field magnetization data was used for calculating the number of active magnetic ions in semiconductor matrix.

查看原文

微信好友朋友圈 QQ好友复制链接

本刊更多论文

Ge1-x-ySixMnyTe多铁质中的类铁磁性相互作用

掺杂磁性杂质的IV-VI材料为自旋电子应用提供了令人兴奋的机会，特别是通过在半导体矩阵中加入存储组件。本文研究了载流子介导的锰离子合金GeTe晶格中的磁相互作用。我们提出了化学成分为Si， x = 0.057, 0.053和Mn， y = 0.035, 0.041的Ge1-x-ySixMnyTe块状晶体，以探索这些晶体中主要的磁相互作用。结果表明，两种晶体的磁相变温度均接近170 K，其中y = 0.035时居里-魏斯温度（θ）为171 K， y = 0.041时居里-魏斯温度（θ）为172.8 K，表明Mn离子之间具有类似铁磁的相互作用。当Mn含量从y = 0.035增加到0.041时，磁化峰的最大值增大了约一个数量级。修正居里-魏斯定律适用于磁化率逆发现合金中的类铁磁相互作用。此外，利用强磁场数据计算了半导体基体中活性磁性离子的数量。

本文章由计算机程序翻译，如有差异，请以英文原文为准。

求助全文

约1分钟内获得全文去求助

来源期刊

Solid State Communications 物理-物理：凝聚态物理

CiteScore

3.40

自引率

4.80%

发文量

287

审稿时长

51 days

期刊介绍： Solid State Communications is an international medium for the publication of short communications and original research articles on significant developments in condensed matter science, giving scientists immediate access to important, recently completed work. The journal publishes original experimental and theoretical research on the physical and chemical properties of solids and other condensed systems and also on their preparation. The submission of manuscripts reporting research on the basic physics of materials science and devices, as well as of state-of-the-art microstructures and nanostructures, is encouraged. A coherent quantitative treatment emphasizing new physics is expected rather than a simple accumulation of experimental data. Consistent with these aims, the short communications should be kept concise and short, usually not longer than six printed pages. The number of figures and tables should also be kept to a minimum. Solid State Communications now also welcomes original research articles without length restrictions. The Fast-Track section of Solid State Communications is the venue for very rapid publication of short communications on significant developments in condensed matter science. The goal is to offer the broad condensed matter community quick and immediate access to publish recently completed papers in research areas that are rapidly evolving and in which there are developments with great potential impact.