Microwave-assisted synthesis of sulfur-doped carbon quantum dots and their application in logic gate operations

Materials Today Quantum Pub Date : 2025-03-01 Epub Date: 2024-12-17 DOI:10.1016/j.mtquan.2024.100021
Lijun Liu , Xiangru Hou , Lu Ga , Yanqing Du , Jun Ai , Gerile Aodeng
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Abstract

In this work, sulfur-doped carbon quantum dots (GSH/L-CyS CQDs) were fabricated using a facile one-step microwave method with reduced glutathione (GSH) and L-cysteine (L-CyS) as the precursors for carbon and sulfur, respectively. The prepared GSH/L-CyS CQDs show high fluorescence signals at 451 nm upon excitation at 375 nm and can selectively detect Co2 + and Ni2+ among various anions and cations. In combination with citric acid (CA), a metal ion masking agent for Ni2+, the IMPLICATION logic gate and NOR logic gate can be operated by controlling different fluorescence inputs and outputs. This research offers a promising avenue for the design and construction of advanced logic gate systems based on CQDs, which may find potential applications in fields such as sensing, computing, and information processing.
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硫掺杂碳量子点的微波辅助合成及其在逻辑门运算中的应用
本文以还原型谷胱甘肽(GSH)和l -半胱氨酸(L-CyS)分别为碳和硫的前体,采用简单的一步微波法制备了硫掺杂碳量子点(GSH/L-CyS)。制备的GSH/L-CyS CQDs在375 nm处激发后,在451 nm处显示出较高的荧光信号,可以选择性检测各种阴离子和阳离子中的Co2 +和Ni2+。与Ni2+的金属离子掩蔽剂柠檬酸(CA)结合,通过控制不同的荧光输入和输出来操作隐含逻辑门和NOR逻辑门。该研究为基于CQDs的高级逻辑门系统的设计和构建提供了一条有希望的途径,它可能在传感、计算和信息处理等领域找到潜在的应用。
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