Rational Design of Three-Dimensional Architectures of Carbon Nanorods/Carbon Nanofibers Composite for High-Performance Supercapacitors

IF 5.5 3区 材料科学 Q2 CHEMISTRY, PHYSICAL ACS Applied Energy Materials Pub Date : 2025-01-16 DOI:10.1021/acsaem.4c03006
Yongsheng Zhou*, Qiuyu Li, Tianyu Lu, Yiyi Zhang, Weibing He, Erhui Zhang, Chuan Liu, Xuchun Wang, Zirong Li, Yingchun Zhu and Bingshe Xu, 
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Abstract

Carbon nanofibers (CNFs) have important application potential in the field of supercapacitors; however, the relatively low specific surface area often leads to a low capacitance. Herein, N-doped carbon nanofibers/carbon nanorods (CNFs/CNRs-N) composite with an N-doping level up to 8.9 atom % is designed, which shows excellent supercapacitor energy storage performance. CNFs/CNRs-N has a three-dimensional porous structure, a large specific surface area, and a huge number of active sites. Based on the synergy of various unique properties of CNFs/CNRs-N, when used as a supercapacitor electrode material, it shows a specific capacitance value of up to 595 F g–1.

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高性能超级电容器用碳纳米棒/碳纳米纤维复合材料三维结构的合理设计
纳米碳纤维在超级电容器领域具有重要的应用潜力;然而,相对较低的比表面积往往导致低电容。本文设计了n掺杂碳纳米纤维/碳纳米棒(CNFs/CNRs-N)复合材料,其n掺杂水平高达8.9原子%,具有优异的超级电容器储能性能。CNFs/CNRs-N具有三维多孔结构、较大的比表面积和大量的活性位点。基于CNFs/CNRs-N各种独特性能的协同作用,当用作超级电容器电极材料时,其比电容值高达595 gf - 1。
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来源期刊
ACS Applied Energy Materials
ACS Applied Energy Materials Materials Science-Materials Chemistry
CiteScore
10.30
自引率
6.20%
发文量
1368
期刊介绍: ACS Applied Energy Materials is an interdisciplinary journal publishing original research covering all aspects of materials, engineering, chemistry, physics and biology relevant to energy conversion and storage. The journal is devoted to reports of new and original experimental and theoretical research of an applied nature that integrate knowledge in the areas of materials, engineering, physics, bioscience, and chemistry into important energy applications.
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