Achieving high energy harvest from a siphon boosted microbial fuel cell-constructed wetland system

IF 6.7 2区 工程技术 Q1 ENGINEERING, CHEMICAL Journal of water process engineering Pub Date : 2025-03-01 Epub Date: 2025-02-12 DOI:10.1016/j.jwpe.2025.107249
Cheng Tang , Yaqian Zhao , Chun Kang , Yanhui Li , David Morgan
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Abstract

Microbial fuel cell-constructed wetland (MFC-CW) coupling system is a kind of bio-electrochemical intensified CW system which upgrades CW into multi-functional wastewater treatment technology. Achieving robust electrical energy output is one of the critical challenges in MFC-CW. However, some critical factors limited power output of MFC-CW in terms of reactions on electrode. These inhibited cathodic reactions were mainly due to insufficient oxygen supporting and great overpotential of anode because of the excessive oxygen diffusion. This study reports a novel siphon containing MFC-CW and its operational strategy (namely a full siphon recirculation (FSR) mode), to boost power output of the MFC-CW. Consecutive tidal flow (TF) cycles were established by FSR in cathode chamber which contributed to the better performances of both the cathode and the anode. Results show that the highest power density, coulombic efficiency (CE) and normalized energy recovery (NER) in FSR mode were 1.15 mW/L, 19.28 %, 128.15 Wh/kg COD, respectively. Power output of MFC-CW with FSR mode were remarkable high and sustainable compared with other MFC-CW studies with normalized assessment criteria. FSR mode simultaneously shows advantages over the high cathode potential and low anode potential. This novel structure and the operation strategy can be regarded as a smart choice to level up power output of MFC-CW system.

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从虹吸推进微生物燃料电池构建的湿地系统实现高能量收获
微生物燃料电池-人工湿地(MFC-CW)耦合系统是一种生物电化学强化的连续水处理系统,将连续水处理提升为多功能污水处理技术。实现稳定的电能输出是MFC-CW的关键挑战之一。然而,一些关键因素限制了MFC-CW在电极上的反应功率输出。这些阴极反应的抑制主要是由于氧支持不足和氧过度扩散导致阳极产生过大的过电位。本研究报告了一种含有MFC-CW的新型虹吸管及其操作策略(即全虹吸管再循环(FSR)模式),以提高MFC-CW的功率输出。FSR在阴极室中建立了连续的潮汐流循环,使阴极和阳极的性能都得到了提高。结果表明,FSR模式下的最高功率密度、库仑效率(CE)和归一化能量回收率(NER)分别为1.15 mW/L、19.28%和128.15 Wh/kg COD。与其他具有标准化评价标准的MFC-CW研究相比,FSR模式的MFC-CW输出功率显著高且可持续。FSR模式同时具有高阴极电位和低阳极电位的优点。这种新颖的结构和运行策略是提高MFC-CW系统输出功率的一种明智选择。
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来源期刊
Journal of water process engineering
Journal of water process engineering Biochemistry, Genetics and Molecular Biology-Biotechnology
CiteScore
10.70
自引率
8.60%
发文量
846
审稿时长
24 days
期刊介绍: The Journal of Water Process Engineering aims to publish refereed, high-quality research papers with significant novelty and impact in all areas of the engineering of water and wastewater processing . Papers on advanced and novel treatment processes and technologies are particularly welcome. The Journal considers papers in areas such as nanotechnology and biotechnology applications in water, novel oxidation and separation processes, membrane processes (except those for desalination) , catalytic processes for the removal of water contaminants, sustainable processes, water reuse and recycling, water use and wastewater minimization, integrated/hybrid technology, process modeling of water treatment and novel treatment processes. Submissions on the subject of adsorbents, including standard measurements of adsorption kinetics and equilibrium will only be considered if there is a genuine case for novelty and contribution, for example highly novel, sustainable adsorbents and their use: papers on activated carbon-type materials derived from natural matter, or surfactant-modified clays and related minerals, would not fulfil this criterion. The Journal particularly welcomes contributions involving environmentally, economically and socially sustainable technology for water treatment, including those which are energy-efficient, with minimal or no chemical consumption, and capable of water recycling and reuse that minimizes the direct disposal of wastewater to the aquatic environment. Papers that describe novel ideas for solving issues related to water quality and availability are also welcome, as are those that show the transfer of techniques from other disciplines. The Journal will consider papers dealing with processes for various water matrices including drinking water (except desalination), domestic, urban and industrial wastewaters, in addition to their residues. It is expected that the journal will be of particular relevance to chemical and process engineers working in the field. The Journal welcomes Full Text papers, Short Communications, State-of-the-Art Reviews and Letters to Editors and Case Studies
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