Impact of sulfur-ash reduction treatment on combustion performance, SOx emissions, and flue gas temperatures of lignite coals: experimental and computational study

IF 5.8 3区 环境科学与生态学 0 ENVIRONMENTAL SCIENCES Environmental Science and Pollution Research Pub Date : 2025-02-12 DOI:10.1007/s11356-025-36064-5
Mansoor Ahmed Lakhmir, Faheem Akhter, Jawad Ahmed, Sidra Mushtaq, Haris Jawad Arain, Muhammad Junaid Ahsan
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Abstract

This study is focused on experimental and computational investigation into effects of sulfur-ash reduction treatment over environmental and simulated combustion behavior of lignite coals, specifically Lakhra and Balochistan coals. The simulative investigation was conducted using computational fluid dynamics (CFD). A 2D CFD model of a coal combustor was developed using Ansys FLUENT to analyze the impact of coal treatment, pressure, and coal feeding rate on sulfur oxide (SOx) generation, combustion efficiency, and temperature profiles. The research aims to provide insights into optimizing coal combustion processes for efficient energy production and reduced environmental impact. The results indicate that treating coal leads to an increase in CO2 and H2O production while reducing CO levels, particularly evident in Balochistan coal. Elevated pressure positively affects combustion efficiency, reflected in higher CO2 and H2O mole fractions. The study also reveals that while combustion efficiency slightly decreases with an increase in coal feeding rate, treated coal exhibits a lesser decrease compared to raw coal. SOx generation is significantly reduced up to 55 to 62% after treatment, reaching negligible levels, with both pressure and coal feeding rate influencing SOx generation. Despite similar sulfur content, Lakhra and Balochistan coals exhibit comparable SOx generation due to their similar sulfur ranges. Temperature profiles show that treated coals exhibit higher temperatures during combustion compared to raw coals, with pressure and coal feeding rate directly influencing temperature. Maximum temperature was found in the range of 2555 to 2564 K. While pressure has a minor positive effect on temperature for Lakhra coal, Balochistan coal shows high sensitivity to pressure. These findings highlight the importance of coal treatment and pressure optimization for reducing SOx emissions and improving combustion efficiency in coal-fired power plants.

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硫灰还原处理对褐煤燃烧性能、硫氧化物排放和烟气温度的影响:实验和计算研究。
本研究的重点是硫灰还原处理对褐煤,特别是拉赫拉和俾路支省煤的环境和模拟燃烧行为的影响的实验和计算研究。利用计算流体力学(CFD)进行了模拟研究。利用Ansys FLUENT软件建立了燃煤燃烧室的二维CFD模型,分析了煤处理、压力和给煤量对硫氧化物(SOx)生成、燃烧效率和温度分布的影响。该研究旨在为优化煤炭燃烧过程提供见解,以实现高效的能源生产和减少对环境的影响。结果表明,煤处理导致CO2和H2O产量增加,同时降低CO水平,特别是在俾路支省的煤中。压力升高对燃烧效率有积极影响,这体现在CO2和H2O摩尔分数的升高上。研究还表明,虽然燃烧效率随着加煤速率的增加而略有下降,但处理后的煤与原煤相比下降幅度较小。处理后的SOx生成显著减少,可达55% ~ 62%,达到可以忽略不计的水平,压力和给煤速率对SOx生成都有影响。尽管含硫量相似,Lakhra和Balochistan的煤由于其相似的硫范围而表现出相似的硫生成。温度分布表明,处理后的煤在燃烧过程中表现出比原煤更高的温度,压力和给煤速度直接影响温度。最高温度范围为2555 ~ 2564 K。虽然压力对拉赫拉煤的温度有轻微的积极影响,但俾路支省的煤对压力表现出高度敏感。这些发现突出了煤处理和压力优化对于减少燃煤电厂硫氧化物排放和提高燃烧效率的重要性。
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来源期刊
CiteScore
8.70
自引率
17.20%
发文量
6549
审稿时长
3.8 months
期刊介绍: Environmental Science and Pollution Research (ESPR) serves the international community in all areas of Environmental Science and related subjects with emphasis on chemical compounds. This includes: - Terrestrial Biology and Ecology - Aquatic Biology and Ecology - Atmospheric Chemistry - Environmental Microbiology/Biobased Energy Sources - Phytoremediation and Ecosystem Restoration - Environmental Analyses and Monitoring - Assessment of Risks and Interactions of Pollutants in the Environment - Conservation Biology and Sustainable Agriculture - Impact of Chemicals/Pollutants on Human and Animal Health It reports from a broad interdisciplinary outlook.
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