Memory and Friction: From the Nanoscale to the Macroscale.

IF 11.7 1区 化学 Q1 CHEMISTRY, PHYSICAL Annual review of physical chemistry Pub Date : 2025-04-01 Epub Date: 2025-02-14 DOI:10.1146/annurev-physchem-082423-031037
Benjamin A Dalton, Anton Klimek, Henrik Kiefer, Florian N Brünig, Hélène Colinet, Lucas Tepper, Amir Abbasi, Roland R Netz
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Abstract

Friction is a phenomenon that manifests across all spatial and temporal scales, from the molecular to the macroscopic scale. It describes the dissipation of energy from the motion of particles or abstract reaction coordinates and arises in the transition from a detailed molecular-level description to a simplified, coarse-grained model. It has long been understood that time-dependent (non-Markovian) friction effects are critical for describing the dynamics of many systems, but that they are notoriously difficult to evaluate for complex physical, chemical, and biological systems. In recent years, the development of advanced numerical friction extraction techniques and methods to simulate the generalized Langevin equation has enabled exploration of the role of time-dependent friction across all scales. We discuss recent applications of these friction extraction techniques and the growing understanding of the role of friction in complex equilibrium and nonequilibrium dynamic many-body systems.

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记忆与摩擦:从纳米尺度到宏观尺度。
从分子到宏观尺度,摩擦是一种跨越所有空间和时间尺度的现象。它描述了粒子运动或抽象反应坐标的能量耗散,并出现在从详细的分子水平描述到简化的粗粒度模型的过渡中。长期以来,人们一直认为,时间依赖(非马尔可夫)摩擦效应对于描述许多系统的动力学至关重要,但对于复杂的物理、化学和生物系统来说,它们是出了名的难以评估的。近年来,先进的数值摩擦提取技术和模拟广义朗之万方程的方法的发展,使得探索时间相关摩擦在所有尺度上的作用成为可能。我们讨论了这些摩擦提取技术的最新应用,以及对摩擦在复杂平衡和非平衡动态多体系统中的作用的日益加深的理解。
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来源期刊
CiteScore
28.00
自引率
0.00%
发文量
21
期刊介绍: The Annual Review of Physical Chemistry has been published since 1950 and is a comprehensive resource for significant advancements in the field. It encompasses various sub-disciplines such as biophysical chemistry, chemical kinetics, colloids, electrochemistry, geochemistry and cosmochemistry, chemistry of the atmosphere and climate, laser chemistry and ultrafast processes, the liquid state, magnetic resonance, physical organic chemistry, polymers and macromolecules, and others.
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