{"title":"Stable Néel-Twisted Skyrmion Bags in a van der Waals Magnet Fe3–xGaTe2 at Room Temperature","authors":"Jialiang Jiang, Yaodong Wu, Lingyao Kong, Yongsen Zhang, Sheng Qiu, Huanhuan Zhang, Yajiao Ke, Shouguo Wang, Mingliang Tian, Jin Tang","doi":"10.1021/acs.nanolett.4c06281","DOIUrl":null,"url":null,"abstract":"Magnetic skyrmion bags with diverse topological charges, <i>Q</i>, offer prospects for future spintronic devices based on freedom of <i>Q</i>, while their emergence in van der Waals magnets holds the potential in developing <i>Q</i>-based 2D topological spintronics. However, previous room temperature skyrmion bags necessitate special anisotropy engineering through disorder Fe intercalation, and the stable phase diagram for skyrmion bags across room temperature regions is lacking. Here, we demonstrate the observation and electrical manipulation of room temperature skyrmion bags in Fe<sub>3–<i>x</i></sub>GaTe<sub>2</sub> without specially designed Fe intercalation. Combining the pulsed currents with the assistance of magnetic fields, skyrmion bags with various topological charges are generated and annihilated. Especially double nested skyrmion bags are also discovered at room temperature. The stable temperature–field diagram of skyrmion bags has been established. We also demonstrate electrically controlled topological phase transformations of skyrmion bags. Our results will provide novel insights for the design of 2D skyrmion-based high-performance devices.","PeriodicalId":53,"journal":{"name":"Nano Letters","volume":"3 1","pages":""},"PeriodicalIF":9.6000,"publicationDate":"2025-02-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Nano Letters","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1021/acs.nanolett.4c06281","RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0
Abstract
Magnetic skyrmion bags with diverse topological charges, Q, offer prospects for future spintronic devices based on freedom of Q, while their emergence in van der Waals magnets holds the potential in developing Q-based 2D topological spintronics. However, previous room temperature skyrmion bags necessitate special anisotropy engineering through disorder Fe intercalation, and the stable phase diagram for skyrmion bags across room temperature regions is lacking. Here, we demonstrate the observation and electrical manipulation of room temperature skyrmion bags in Fe3–xGaTe2 without specially designed Fe intercalation. Combining the pulsed currents with the assistance of magnetic fields, skyrmion bags with various topological charges are generated and annihilated. Especially double nested skyrmion bags are also discovered at room temperature. The stable temperature–field diagram of skyrmion bags has been established. We also demonstrate electrically controlled topological phase transformations of skyrmion bags. Our results will provide novel insights for the design of 2D skyrmion-based high-performance devices.
期刊介绍:
Nano Letters serves as a dynamic platform for promptly disseminating original results in fundamental, applied, and emerging research across all facets of nanoscience and nanotechnology. A pivotal criterion for inclusion within Nano Letters is the convergence of at least two different areas or disciplines, ensuring a rich interdisciplinary scope. The journal is dedicated to fostering exploration in diverse areas, including:
- Experimental and theoretical findings on physical, chemical, and biological phenomena at the nanoscale
- Synthesis, characterization, and processing of organic, inorganic, polymer, and hybrid nanomaterials through physical, chemical, and biological methodologies
- Modeling and simulation of synthetic, assembly, and interaction processes
- Realization of integrated nanostructures and nano-engineered devices exhibiting advanced performance
- Applications of nanoscale materials in living and environmental systems
Nano Letters is committed to advancing and showcasing groundbreaking research that intersects various domains, fostering innovation and collaboration in the ever-evolving field of nanoscience and nanotechnology.