Stable Néel-Twisted Skyrmion Bags in a van der Waals Magnet Fe3–xGaTe2 at Room Temperature

IF 9.1 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY Nano Letters Pub Date : 2025-02-17 DOI:10.1021/acs.nanolett.4c06281
Jialiang Jiang, Yaodong Wu, Lingyao Kong, Yongsen Zhang, Sheng Qiu, Huanhuan Zhang, Yajiao Ke, Shouguo Wang, Mingliang Tian, Jin Tang
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Abstract

Magnetic skyrmion bags with diverse topological charges, Q, offer prospects for future spintronic devices based on freedom of Q, while their emergence in van der Waals magnets holds the potential in developing Q-based 2D topological spintronics. However, previous room temperature skyrmion bags necessitate special anisotropy engineering through disorder Fe intercalation, and the stable phase diagram for skyrmion bags across room temperature regions is lacking. Here, we demonstrate the observation and electrical manipulation of room temperature skyrmion bags in Fe3–xGaTe2 without specially designed Fe intercalation. Combining the pulsed currents with the assistance of magnetic fields, skyrmion bags with various topological charges are generated and annihilated. Especially double nested skyrmion bags are also discovered at room temperature. The stable temperature–field diagram of skyrmion bags has been established. We also demonstrate electrically controlled topological phase transformations of skyrmion bags. Our results will provide novel insights for the design of 2D skyrmion-based high-performance devices.

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室温下范德华磁体Fe3-xGaTe2中稳定的nsamel - twisted Skyrmion Bags
具有不同拓扑电荷Q的磁skyrmion袋为未来基于Q自由度的自旋电子器件提供了前景,而它们在范德华磁体中的出现为发展基于Q的二维拓扑自旋电子学提供了潜力。然而,以往的常温skyrmion袋需要通过无序Fe插层进行特殊的各向异性工程,并且缺乏skyrmion袋跨室温区域的稳定相图。在这里,我们展示了在没有特别设计的Fe嵌入的情况下,在Fe3-xGaTe2中观察和电操作室温skyrmion袋。结合脉冲电流和磁场的辅助,产生并湮灭了具有各种拓扑电荷的粒子袋。特别是在室温下也发现了双层嵌套的skyrmion袋。建立了丝瓜袋的稳定温度场图。我们还演示了电控制的skyrmion袋的拓扑相变。我们的研究结果将为基于二维skyrion的高性能器件的设计提供新的见解。
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来源期刊
Nano Letters
Nano Letters 工程技术-材料科学:综合
CiteScore
16.80
自引率
2.80%
发文量
1182
审稿时长
1.4 months
期刊介绍: Nano Letters serves as a dynamic platform for promptly disseminating original results in fundamental, applied, and emerging research across all facets of nanoscience and nanotechnology. A pivotal criterion for inclusion within Nano Letters is the convergence of at least two different areas or disciplines, ensuring a rich interdisciplinary scope. The journal is dedicated to fostering exploration in diverse areas, including: - Experimental and theoretical findings on physical, chemical, and biological phenomena at the nanoscale - Synthesis, characterization, and processing of organic, inorganic, polymer, and hybrid nanomaterials through physical, chemical, and biological methodologies - Modeling and simulation of synthetic, assembly, and interaction processes - Realization of integrated nanostructures and nano-engineered devices exhibiting advanced performance - Applications of nanoscale materials in living and environmental systems Nano Letters is committed to advancing and showcasing groundbreaking research that intersects various domains, fostering innovation and collaboration in the ever-evolving field of nanoscience and nanotechnology.
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