Room Temperature Broadband Polariton Lasing from a CsPbBr3 Perovskite Plate

IF 8 2区 材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Advanced Optical Materials Pub Date : 2024-12-31 DOI:10.1002/adom.202402543
Maksim D. Kolker, Ivan I. Krasionov, Anton D. Putintsev, Ekaterina D. Grayfer, Tamsin Cookson, Dmitry Tatarinov, Anatoly P. Pushkarev, Denis A. Sannikov, Pavlos G. Lagoudakis
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Abstract

Tunable polariton lasing is demonstrated from an all-inorganic CsPbBr3 perovskite microcrystal plate over 23 nm in the green part of the optical spectrum, operating at room temperature. The emission spectrum is controlled by adjusting the effective length of a multi- λ $\bm{\lambda }$ planar microcavity, whilst observing the hallmarks of polariton condensation under non-resonant excitation. Furthermore, simultaneous condensation is observed into two non-degenerate lower polariton branches of orthogonal polarizations induced by anisotropy of the perovskite crystal.

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在室温下工作时,从全无机 CsPbBr3 包晶石微晶板上展示了 23 nm 以上的可调偏振子激光,其光谱为绿色部分。通过调节多 λ $bm{\lambda }$ 平面微腔的有效长度控制了发射光谱,同时观察到了非共振激发下的极化子凝聚特征。此外,还观察到在过氧化物晶体各向异性的诱导下,同时凝聚成两个正交极化的非退化下极化子分支。
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来源期刊
Advanced Optical Materials
Advanced Optical Materials MATERIALS SCIENCE, MULTIDISCIPLINARY-OPTICS
CiteScore
13.70
自引率
6.70%
发文量
883
审稿时长
1.5 months
期刊介绍: Advanced Optical Materials, part of the esteemed Advanced portfolio, is a unique materials science journal concentrating on all facets of light-matter interactions. For over a decade, it has been the preferred optical materials journal for significant discoveries in photonics, plasmonics, metamaterials, and more. The Advanced portfolio from Wiley is a collection of globally respected, high-impact journals that disseminate the best science from established and emerging researchers, aiding them in fulfilling their mission and amplifying the reach of their scientific discoveries.
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