Optical Spin Hall Effect Pattern Switching in Polariton Condensates in Organic Single-Crystal Microbelts

IF 15.6 1区 化学 Q1 CHEMISTRY, MULTIDISCIPLINARY Journal of the American Chemical Society Pub Date : 2025-02-26 DOI:10.1021/jacs.4c15894
Jiahuan Ren, Teng Long, Chunling Gu, Hongbing Fu, Dmitry Solnyshkov, Guillaume Malpuech, Qing Liao
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Abstract

Topological polaritons, combining the robustness of the topologically protected edge states against defects and disorder with the strong nonlinear properties of polariton bosons, represent an excellent platform to investigate novel photonic topological phases. We demonstrate the optical spin Hall effect (OSHE) and its symmetry switching in the exciton–polariton regime of pure DPAVBi crystals. Benefiting from the photonic Rashba–Dresselhaus spin–orbit coupling, we observe the separation of left- and right-circularly polarized emission in momentum space and real space, a signature of the OSHE. Above the lasing threshold, the OSHE pattern changes due to transverse quantization in the microbelt. This simple device has great potential applications in topological polaritons, such as information transmission, photonic integrated chips, and quantum information.

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有机单晶微带中极化子凝聚体的光自旋霍尔效应模式切换
拓扑极化子结合了拓扑保护边缘态对缺陷和无序的鲁棒性以及极化子玻色子的强非线性特性,为研究新的光子拓扑相提供了一个很好的平台。研究了纯DPAVBi晶体在激子-极化态下的光自旋霍尔效应(OSHE)及其对称开关。利用光子Rashba-Dresselhaus自旋-轨道耦合,我们观察到在动量空间和实空间中左右圆极化发射的分离,这是OSHE的一个特征。在激光阈值以上,由于微带中的横向量化,OSHE模式发生了变化。这种简单的器件在拓扑极化,如信息传输、光子集成芯片、量子信息等方面有很大的应用潜力。
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来源期刊
CiteScore
24.40
自引率
6.00%
发文量
2398
审稿时长
1.6 months
期刊介绍: The flagship journal of the American Chemical Society, known as the Journal of the American Chemical Society (JACS), has been a prestigious publication since its establishment in 1879. It holds a preeminent position in the field of chemistry and related interdisciplinary sciences. JACS is committed to disseminating cutting-edge research papers, covering a wide range of topics, and encompasses approximately 19,000 pages of Articles, Communications, and Perspectives annually. With a weekly publication frequency, JACS plays a vital role in advancing the field of chemistry by providing essential research.
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