{"title":"Optical Spin Hall Effect Pattern Switching in Polariton Condensates in Organic Single-Crystal Microbelts","authors":"Jiahuan Ren, Teng Long, Chunling Gu, Hongbing Fu, Dmitry Solnyshkov, Guillaume Malpuech, Qing Liao","doi":"10.1021/jacs.4c15894","DOIUrl":null,"url":null,"abstract":"Topological polaritons, combining the robustness of the topologically protected edge states against defects and disorder with the strong nonlinear properties of polariton bosons, represent an excellent platform to investigate novel photonic topological phases. We demonstrate the optical spin Hall effect (OSHE) and its symmetry switching in the exciton–polariton regime of pure DPAVBi crystals. Benefiting from the photonic Rashba–Dresselhaus spin–orbit coupling, we observe the separation of left- and right-circularly polarized emission in momentum space and real space, a signature of the OSHE. Above the lasing threshold, the OSHE pattern changes due to transverse quantization in the microbelt. This simple device has great potential applications in topological polaritons, such as information transmission, photonic integrated chips, and quantum information.","PeriodicalId":49,"journal":{"name":"Journal of the American Chemical Society","volume":"25 1","pages":""},"PeriodicalIF":14.4000,"publicationDate":"2025-02-26","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Journal of the American Chemical Society","FirstCategoryId":"92","ListUrlMain":"https://doi.org/10.1021/jacs.4c15894","RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0
Abstract
Topological polaritons, combining the robustness of the topologically protected edge states against defects and disorder with the strong nonlinear properties of polariton bosons, represent an excellent platform to investigate novel photonic topological phases. We demonstrate the optical spin Hall effect (OSHE) and its symmetry switching in the exciton–polariton regime of pure DPAVBi crystals. Benefiting from the photonic Rashba–Dresselhaus spin–orbit coupling, we observe the separation of left- and right-circularly polarized emission in momentum space and real space, a signature of the OSHE. Above the lasing threshold, the OSHE pattern changes due to transverse quantization in the microbelt. This simple device has great potential applications in topological polaritons, such as information transmission, photonic integrated chips, and quantum information.
期刊介绍:
The flagship journal of the American Chemical Society, known as the Journal of the American Chemical Society (JACS), has been a prestigious publication since its establishment in 1879. It holds a preeminent position in the field of chemistry and related interdisciplinary sciences. JACS is committed to disseminating cutting-edge research papers, covering a wide range of topics, and encompasses approximately 19,000 pages of Articles, Communications, and Perspectives annually. With a weekly publication frequency, JACS plays a vital role in advancing the field of chemistry by providing essential research.