Sonocatalytical Nanoparticles with Persistent Action after Ceasing Ultrasound for Water Disinfection

Zeinab Marfavi, Yijun Han, Yuhao Cai, Quanjie Lv, Kang Sun, Congli Yuan and Ke Tao*, 
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Abstract

Efficient water contaminant removal is critical for ecological and environmental sustainability. Developing energy-efficient, cost-effective catalysts compatible with existing water treatment systems is essential. This study introduces NdYVO4:Eu3+ nanoparticles as promising sonocatalysts, capable of generating reactive oxygen species (ROS) during ultrasound (US) exposure and maintaining persistent ROS activity for up to 12 h postexposure. These nanoparticles effectively degraded methylene orange and rhodamine B and demonstrated significant antibacterial efficacy against Staphylococcus aureus and Escherichia coli. The findings were further validated by using nanoparticle-coated industrial ceramic plates. This work provides an alternative procedure for US-triggered ROS production and suggests that NdYVO4:Eu3+ nanoparticles might be promising in sonocatalytic water treatment.

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水消毒停止超声后具有持续作用的声催化纳米颗粒
有效去除水污染物对生态和环境的可持续性至关重要。开发与现有水处理系统兼容的节能、低成本的催化剂至关重要。这项研究介绍了NdYVO4:Eu3+纳米颗粒作为有前途的声催化剂,能够在超声(US)暴露期间产生活性氧(ROS),并在暴露后12小时内保持持续的ROS活性。这些纳米颗粒能有效降解亚甲基橙和罗丹明B,并对金黄色葡萄球菌和大肠杆菌具有显著的抗菌作用。利用纳米颗粒涂覆的工业陶瓷板进一步验证了这一发现。这项工作为us触发的ROS生产提供了一种替代方法,并表明NdYVO4:Eu3+纳米颗粒在声催化水处理中可能很有前景。
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期刊介绍: ACS Applied Engineering Materials is an international and interdisciplinary forum devoted to original research covering all aspects of engineered materials complementing the ACS Applied Materials portfolio. Papers that describe theory simulation modeling or machine learning assisted design of materials and that provide new insights into engineering applications are welcomed. The journal also considers experimental research that includes novel methods of preparing characterizing and evaluating new materials designed for timely applications. With its focus on innovative applications ACS Applied Engineering Materials also complements and expands the scope of existing ACS publications that focus on materials science discovery including Biomacromolecules Chemistry of Materials Crystal Growth & Design Industrial & Engineering Chemistry Research Inorganic Chemistry Langmuir and Macromolecules.The scope of ACS Applied Engineering Materials includes high quality research of an applied nature that integrates knowledge in materials science engineering physics mechanics and chemistry.
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