{"title":"Effect of applied magnetic field on the complex permeability of polycrystalline Perovskite La0.7Sr0.3-xKxMnO3 (0 ≤ x ≤ 0.15)","authors":"Hsiao-Wen Yu, Fung Jung Liu, YuShan Huang","doi":"10.1016/j.jmmm.2025.172894","DOIUrl":null,"url":null,"abstract":"<div><div>The phase transition temperature and permeability spectra under magnetic fields for polycrystalline La<sub>0.7</sub>Sr<sub>0.3-</sub><em><sub>x</sub></em>K<em><sub>x</sub></em>MnO<sub>3</sub> (0 ≤ <em>x</em> ≤ 0.15) were measured. All samples exhibited ferromagnetic–paramagnetic and corresponding metallic-insulating phase transitions. As the concentration of K<sup>+</sup> ion increased, the phase transition temperature decreased. The relative complex permeability <em>μ<sub>r</sub></em> = <em>μ<sub>r</sub>′</em> − <em>jμ<sub>r</sub>′′</em> in the range of 10 kHz-13 MHz was investigated under an applied DC magnetic field <em>B<sub>dc</sub></em>. All measured magnetic spectra showed relaxation behavior due to domain wall displacement. As the doping concentration <em>x</em> increased, the permeability decreased, and the relaxation frequency <em>f<sub>r</sub></em> increased. Under <em>B<sub>dc</sub></em>, the amount of <em>f<sub>r</sub></em> increased rapidly. The slope of the <em>f<sub>r</sub></em> v.s. <em>B<sub>dc</sub></em> curve, defined as the magnetic field-to-frequency transfer ratio Δ<em>f<sub>r</sub></em>/Δ<em>B<sub>dc</sub></em>, was enhanced by potassium doping. The highest Δ<em>f<sub>r</sub></em>/Δ<em>B<sub>dc</sub></em> value (=1.89 kHz/Oe) was observed for the <em>x</em> = 0.15 sample. The significant change in <em>f<sub>r</sub></em> under <em>B<sub>dc</sub></em> shows promise for magnetic sensor applications.</div></div>","PeriodicalId":366,"journal":{"name":"Journal of Magnetism and Magnetic Materials","volume":"620 ","pages":"Article 172894"},"PeriodicalIF":2.5000,"publicationDate":"2025-02-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Journal of Magnetism and Magnetic Materials","FirstCategoryId":"88","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S0304885325001258","RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0
Abstract
The phase transition temperature and permeability spectra under magnetic fields for polycrystalline La0.7Sr0.3-xKxMnO3 (0 ≤ x ≤ 0.15) were measured. All samples exhibited ferromagnetic–paramagnetic and corresponding metallic-insulating phase transitions. As the concentration of K+ ion increased, the phase transition temperature decreased. The relative complex permeability μr = μr′ − jμr′′ in the range of 10 kHz-13 MHz was investigated under an applied DC magnetic field Bdc. All measured magnetic spectra showed relaxation behavior due to domain wall displacement. As the doping concentration x increased, the permeability decreased, and the relaxation frequency fr increased. Under Bdc, the amount of fr increased rapidly. The slope of the fr v.s. Bdc curve, defined as the magnetic field-to-frequency transfer ratio Δfr/ΔBdc, was enhanced by potassium doping. The highest Δfr/ΔBdc value (=1.89 kHz/Oe) was observed for the x = 0.15 sample. The significant change in fr under Bdc shows promise for magnetic sensor applications.
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