Eddy covariance towers as sentinels of abnormal radioactive material releases

IF 5.8 3区 环境科学与生态学 0 ENVIRONMENTAL SCIENCES Environmental Science and Pollution Research Pub Date : 2025-02-27 DOI:10.1007/s11356-025-36171-3
Jemma Stachelek, Lee Turin Dickman, Vachel A. Kraklow, Emily Casleton, Elizabeth Christi Thompson, Sanna Sevanto, Ann Junghans
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Abstract

Ensuring accurate detection and attribution of abnormal releases of radioactive material is critical for protecting human health and safety. Most commonly, such detection is accomplished via active monitoring approaches involving the collection of physical samples. This is labor intensive and limits the temporal and spatial resolution of any detected events to a relatively coarse level. As an alternative first step towards passive monitoring, we developed an approach using eddy flux tower data records to identify signals from a known abnormal release and quantify the extent to which that signal also occurs at other times in the data record. Through two case studies, one of which targeted the Fukushima nuclear disaster and the other targeting an abnormal release event at a radioisotope production facility in Fleurus, Belgium, we tested our approach and identified several potential heretofore unidentified abnormal events that were consistent with atmospheric circulation patterns and/or wind direction from known release sites. Because our approach is relatively simple and is resistant to systematic errors in the observational record, it has broad applicability beyond specific constituents and ecosystem types to identify a wide variety of limited-duration anomalies in flux tower data to ensure human health and industrial safety.

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涡旋相关塔是异常放射性物质释放的哨兵。
确保准确探测和查明放射性物质异常释放的原因,对于保护人类健康和安全至关重要。最常见的是,这种检测是通过主动监测方法完成的,包括收集物理样本。这是劳动密集型的,并且将任何检测到的事件的时间和空间分辨率限制在相对粗糙的水平。作为被动监测的第一步,我们开发了一种方法,使用涡流通量塔数据记录来识别已知异常释放的信号,并量化该信号在数据记录中其他时间发生的程度。通过两个案例研究,一个是针对福岛核灾难,另一个是针对比利时Fleurus放射性同位素生产设施的异常释放事件,我们测试了我们的方法,并确定了几个潜在的迄今为止未确定的异常事件,这些异常事件与已知释放地点的大气环流模式和/或风向一致。由于我们的方法相对简单,并且能够抵抗观测记录中的系统误差,因此它具有广泛的适用性,超出了特定成分和生态系统类型,可以识别通量塔数据中各种有限持续时间的异常,以确保人类健康和工业安全。
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来源期刊
CiteScore
8.70
自引率
17.20%
发文量
6549
审稿时长
3.8 months
期刊介绍: Environmental Science and Pollution Research (ESPR) serves the international community in all areas of Environmental Science and related subjects with emphasis on chemical compounds. This includes: - Terrestrial Biology and Ecology - Aquatic Biology and Ecology - Atmospheric Chemistry - Environmental Microbiology/Biobased Energy Sources - Phytoremediation and Ecosystem Restoration - Environmental Analyses and Monitoring - Assessment of Risks and Interactions of Pollutants in the Environment - Conservation Biology and Sustainable Agriculture - Impact of Chemicals/Pollutants on Human and Animal Health It reports from a broad interdisciplinary outlook.
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