Advanced Temperature-Integrated Backpropagation Neural Network for Enhanced Prediction of Syngas Composition in Complex Organic Waste Gasification.

Chem & Bio Engineering Pub Date : 2024-11-26 eCollection Date: 2025-02-27 DOI:10.1021/cbe.4c00146
Mingyue Yan, Huiyang Bi, HuanXu Wang, Caicai Xu, Lihao Chen, Lei Zhang, Shuangwei Chen, Xuming Xu, Zhongjian Li, Yang Hou, Lecheng Lei, Bin Yang
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Abstract

Accurate prediction of syngas compositions in multicomponent organic waste gasification is challenging because of its intricate composition and abundant volatile matter, which contrasts with traditional coal gasification influenced mainly by oxygen-coal ratio. Through process analysis, we identified the furnace temperature as a crucial factor directly impacting gasification reactions. Herein, we developed a hybrid backpropagation neural network (BPNN) model integrating furnace temperature data obtained from a temperature soft-sensing model and utilizing principal component analysis (PCA) for dimensionality reduction. The resulting T-PCA-BPNN model demonstrated outstanding predictive performance, achieving R 2 values of 0.95, 0.97, and 0.94 for CO2, CO, and H2, respectively. Compared to the base BPNN model, the total mean square error (MSE) and mean absolute error (MAE) decreased by 49.4% and 13.3%, respectively. Furthermore, the percentage of predictive errors within 1% (QR) surpassed 90%, underscoring the model's practical applicability. Leveraging PCA and SHapley Additive exPlanations (SHAP) analysis, we established a syngas regulation strategy that controls critical parameters to identify postdimensionality reduction through practical operational adjustments. This data-driven model enhances syngas prediction, thereby facilitating improved process control and optimization in complex organic waste gasification.

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先进的温度集成反向传播神经网络用于复杂有机废物气化合成气成分的增强预测。
与传统煤气化主要受氧煤比影响不同,多组分有机废弃物气化过程中合成气组成复杂,挥发分丰富,对合成气成分的准确预测具有一定的挑战性。通过工艺分析,确定了炉温是直接影响气化反应的关键因素。在此,我们开发了一个混合反向传播神经网络(BPNN)模型,该模型集成了从温度软测量模型获得的炉温数据,并利用主成分分析(PCA)进行降维。所得到的T-PCA-BPNN模型表现出出色的预测性能,对CO2、CO和H2的r2值分别为0.95、0.97和0.94。与基本BPNN模型相比,总均方误差(MSE)和平均绝对误差(MAE)分别下降了49.4%和13.3%。预测误差在1%以内(QR)的比例超过90%,表明了模型的实际适用性。利用主成分分析和SHapley加性解释(SHAP)分析,我们建立了一个合成气调节策略,该策略控制关键参数,通过实际操作调整来识别后维数降低。这种数据驱动的模型增强了合成气预测,从而促进了复杂有机废物气化过程控制和优化。
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