Swelling behavior of Cr16Ni19 steel under neutron irradiation: experimental and theoretical analysis

IF 3.2 2区 工程技术 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Journal of Nuclear Materials Pub Date : 2025-05-01 Epub Date: 2025-03-23 DOI:10.1016/j.jnucmat.2025.155771
Alexey Yanilkin , Alexander Kozlov , Irina Portnykh
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Abstract

This paper investigates the swelling behavior of Cr16Ni19 austenitic steel used for fuel cladding in the BN-600 reactor. Experimental investigations were conducted over doses of 0.3–48.5 dpa and temperatures of 370–410 °C using high-resolution electron microscopy, which revealed the formation of helium-vacancy bubbles (∼1.5 nm, 1–3·1022 m−3) and, at doses above 5 dpa, voids exceeding 10 nm in diameter. Dislocation density measurements ranged from (3.4–5)· 1014 m−2, increasing to 7·1014 m−2 at lower irradiation temperatures. A kinetic swelling model was then parameterized using these data, along with high-dose measurements (>50 dpa), to predict swelling behavior and compare it with that of AISI 316 steel. The model suggests that Cr16Ni19 steel exhibits enhanced swelling resistance due to a stable dislocation network and a higher concentration of interstitial clusters, likely influenced by its silicon content. Conventional approximation methods were found to underestimate the fuel element's remaining service life, highlighting the need for predictive models that incorporate real time microstructural data.

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中子辐照下Cr16Ni19钢的膨胀行为:实验与理论分析
研究了BN-600反应堆燃料包壳用Cr16Ni19奥氏体钢的膨胀行为。实验研究在0.3-48.5 dpa和370-410°C的温度下进行,使用高分辨率电子显微镜,发现氦空位气泡(~ 1.5 nm, 1-3·1022 m−3)的形成,在5 dpa以上的剂量下,空洞直径超过10 nm。位错密度的测量范围为(3.4-5)·1014 m−2,在较低的辐照温度下增加到7·1014 m−2。然后,利用这些数据和高剂量测量(50 dpa)参数化动力学膨胀模型,预测膨胀行为,并将其与AISI 316钢进行比较。该模型表明,Cr16Ni19钢具有稳定的位错网络和更高浓度的间隙团簇,这可能受其硅含量的影响,因此具有更强的抗膨胀性。研究发现,传统的近似方法低估了燃料元件的剩余使用寿命,这凸显了对包含实时微观结构数据的预测模型的需求。
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来源期刊
Journal of Nuclear Materials
Journal of Nuclear Materials 工程技术-材料科学:综合
CiteScore
5.70
自引率
25.80%
发文量
601
审稿时长
63 days
期刊介绍: The Journal of Nuclear Materials publishes high quality papers in materials research for nuclear applications, primarily fission reactors, fusion reactors, and similar environments including radiation areas of charged particle accelerators. Both original research and critical review papers covering experimental, theoretical, and computational aspects of either fundamental or applied nature are welcome. The breadth of the field is such that a wide range of processes and properties in the field of materials science and engineering is of interest to the readership, spanning atom-scale processes, microstructures, thermodynamics, mechanical properties, physical properties, and corrosion, for example. Topics covered by JNM Fission reactor materials, including fuels, cladding, core structures, pressure vessels, coolant interactions with materials, moderator and control components, fission product behavior. Materials aspects of the entire fuel cycle. Materials aspects of the actinides and their compounds. Performance of nuclear waste materials; materials aspects of the immobilization of wastes. Fusion reactor materials, including first walls, blankets, insulators and magnets. Neutron and charged particle radiation effects in materials, including defects, transmutations, microstructures, phase changes and macroscopic properties. Interaction of plasmas, ion beams, electron beams and electromagnetic radiation with materials relevant to nuclear systems.
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