Superconductivity in platinum-intercalated 2H-TaS2

IF 6.4 1区 化学 Q1 CHEMISTRY, INORGANIC & NUCLEAR Inorganic Chemistry Frontiers Pub Date : 2025-04-16 DOI:10.1039/D5QI00683J
Lijia Zhou, Xiangjiang Dong, Qiang Li and Xianran Xing
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Abstract

We systematically investigated the superconducting properties of 2H-PtxTaS2 (0 ≤ x ≤ 0.12). As the platinum (Pt) content increases, the charge density wave (CDW) in 2H-TaS2, which appears at approximately 75 K, is progressively suppressed and completely disappears in 2H-Pt0.06TaS2. Meanwhile, the superconducting transition temperature (Tc) first increases and then decreases, reaching its maximum value of approximately 4.85 K at x = 0.06. This phenomenon suggests a competitive interplay between CDW and superconductivity (SC) in this system. Further measurements of the superconducting parameters of 2H-Pt0.06TaS2 indicate that the enhancement of Tc is primarily attributed to an increase in the density of states at the Fermi level.

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铂插层2h - ta2中的超导性
我们系统地研究了2H-PtxTaS2(0≤x≤0.08)的超导性能。随着铂(Pt)含量的增加,2H-TaS2中出现在75 K左右的电荷密度波(CDW)逐渐被抑制,并在Pt0.06TaS2中完全消失。同时,超导转变温度(Tc)先升高后降低,在x = 0.06时达到最大值,约为4.85 K。这一现象表明CDW与超导性(SC)之间存在竞争性相互作用。对Pt0.06TaS2超导参数的进一步测量表明,Tc的增强主要归因于费米能级态密度的增加。
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来源期刊
Inorganic Chemistry Frontiers
Inorganic Chemistry Frontiers CHEMISTRY, INORGANIC & NUCLEAR-
CiteScore
10.40
自引率
7.10%
发文量
587
审稿时长
1.2 months
期刊介绍: The international, high quality journal for interdisciplinary research between inorganic chemistry and related subjects
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