Optimizing integration strategies for biomass gasification with natural gas pyrolysis under a low-carbon hydrogen enhancement approach: A financial and environmental perspective

IF 4.3 2区 工程技术 Q2 ENGINEERING, CHEMICAL Chemical Engineering Science Pub Date : 2025-06-15 Epub Date: 2025-04-18 DOI:10.1016/j.ces.2025.121654
Weiqing Diao, Yi An, Qin Wang
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Abstract

Integrating low-carbon hydrogen through “hydrogen enhancement” can notably increase carbon conversion efficiency in alcohol-based product synthesis, with potential improvements up to nearly double the typical rate. Producing low-carbon hydrogen via a natural gas pyrolysis system (NG-PS) offers a more economically viable approach compared to water electrolysis. This study evaluates and optimized strategies for incorporating natural gas pyrolysis into biomass-to-fuel conversion processes, focusing on the use of Rice Husk biomass as a case study for alcohol-based fuel production. The examined method includes Synthesis gas combustion, NG combustion, H2 combustion, internal heat integration, and electrical heating to supply the necessary heat for pyrolysis. The analysis provides both technoeconomic and greenhouse gas (GHG) emission assessments. Results show that hydrogen-enhanced biomass use in fuel production can reduce GHG emissions by 81% based on a 100-year global warming potential (GWP), and by 72% based on a 20-year GWP, compared to conventional natural gas-based production methods.
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基于低碳氢强化方法的生物质气化与天然气热解优化整合策略:财务和环境视角
通过“增氢”整合低碳氢可以显著提高醇基产品合成中的碳转化效率,其潜在改进率几乎是典型速率的两倍。与水电解相比,通过天然气热解系统(NG-PS)生产低碳氢提供了一种更经济可行的方法。本研究评估并优化了将天然气热解纳入生物质-燃料转化过程的策略,重点研究了稻壳生物质作为酒精基燃料生产的案例研究。考察方法包括合成气燃烧、天然气燃烧、氢气燃烧、内热集成、电加热等,为热解提供必要的热量。该分析提供了技术经济和温室气体(GHG)排放评估。结果表明,与传统的天然气生产方法相比,基于100年全球变暖潜势(GWP)的燃料生产中氢增强生物质的使用可以减少81%的温室气体排放,基于20年全球变暖潜势(GWP)的温室气体排放减少72%。
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来源期刊
Chemical Engineering Science
Chemical Engineering Science 工程技术-工程:化工
CiteScore
7.50
自引率
8.50%
发文量
1025
审稿时长
50 days
期刊介绍: Chemical engineering enables the transformation of natural resources and energy into useful products for society. It draws on and applies natural sciences, mathematics and economics, and has developed fundamental engineering science that underpins the discipline. Chemical Engineering Science (CES) has been publishing papers on the fundamentals of chemical engineering since 1951. CES is the platform where the most significant advances in the discipline have ever since been published. Chemical Engineering Science has accompanied and sustained chemical engineering through its development into the vibrant and broad scientific discipline it is today.
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