Health risk assessment and morphometric study of metal bounded ultrafine aerosol in indo-gangetic plain, India

IF 1.8 4区 地球科学 Q2 ENVIRONMENTAL SCIENCES Journal of Atmospheric Chemistry Pub Date : 2025-04-21 DOI:10.1007/s10874-025-09471-8
Rahul Tiwari, Kalpana Rajouriya, Renuka Saini, Prabal P. Singh, Ajay Taneja
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Abstract

Traffic activities and road dust are major contributors to the release of metals in ambient air which further cause serious health risks by entering the body. This study examined size-segregated PM concentration trends in rural site (Iradatnagar) Risk assessement and disease estimation was done by AirQ + and USEPA Methodology. PM2.5-1.0 levels were 294.64 µg/m³ in summer and 78.81 µg/m³ was found in monsoon, while PM1.0-0.5 measured 204.53 µg/m³ in summer and 66.42 µg/m³ in monsoon, respectively. Al, Ba, Ca, Fe, Mg, Mn, Pb, Ni, Cr, Cd, Cu, and Zn were analyzed. Total metal concentration was found to be 32.96 µg/m3 in summer and 12.27 µg/m3 in monsoon for PM2.5−1.0, while for PM1.0−0.5 it was found as 30.42 µg/m3 and 10.56 µg/m3 in summer and monsson respectively. According to the findings, the concentration of metals was higher in summer. Metal BI ranged from 5.12 to 6.46% (PM2.5-1.0) and 4.56–7.05% (PM1.0-0.5). HQ outcomes Cr(2.78, 9.59E-02), Ni(2.73, 6.85E-01), Al(1.43, 4.79E-01), and Mn(0.19, 1.92E-01) were observed for PM2.5−1.0 in the summer and monsoon seasons respectively. HQ outcomes Cr(3.16, 9.59E-02), Ni(0.68, 6.85E-01), Al(1.55, 5.56E-01), and Mn(0.76, 1.92E-01) were identified for PM1.0−0.5 in summer, and monsoon seasons. HQ was observed higher for PM1.0−0.5 (1.95) size fractions compared to PM2.5−1.0 (1.30). ELCR value for Cr(VI) was found higher for adult in comparison with child whereas the trend followed as as Cr(VI) (0.0007), (0.0002) > Pb (3.52E-06)(1.05E-06) > Ni (1.31E-06)(3.94E-07). Adult values were found to be greater (0.0002) than child values (7.10E-05). The Cancerous risk mean value found two times higher than the permissible limit (1 × 10− 6).

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印度印度河流域平原金属超细气溶胶的健康风险评估和形态计量学研究
交通活动和道路粉尘是环境空气中金属释放的主要因素,金属进入人体进一步造成严重的健康风险。采用AirQ +和USEPA方法进行风险评估和疾病估计。夏季PM2.5-1.0浓度为294.64µg/m³,季风期为78.81µg/m³;夏季PM1.0-0.5浓度为204.53µg/m³,季风期为66.42µg/m³。分析了Al、Ba、Ca、Fe、Mg、Mn、Pb、Ni、Cr、Cd、Cu和Zn。PM2.5−1.0夏季和季候风的总金属浓度分别为32.96µg/m3和12.27µg/m3, PM1.0−0.5夏季和季候风的总金属浓度分别为30.42µg/m3和10.56µg/m3。根据调查结果,金属浓度在夏季较高。金属BI范围为5.12 ~ 6.46% (PM2.5-1.0)和4.56 ~ 7.05% (PM1.0-0.5)。PM2.5−1.0在夏季和季风季节分别观测到Cr(2.78, 9.59E-02)、Ni(2.73, 6.85E-01)、Al(1.43, 4.79E-01)和Mn(0.19, 1.92E-01)的HQ结果。夏季和季风季节PM1.0 - 0.5的HQ结果分别为Cr(3.16, 9.59E-02)、Ni(0.68, 6.85E-01)、Al(1.55, 5.56E-01)和Mn(0.76, 1.92E-01)。与PM2.5 - 1.0(1.30)相比,PM1.0 - 0.5(1.95)颗粒的HQ更高。Cr(VI)的ELCR值成人高于儿童,Cr(VI)(0.0007)、(0.0002)和gt; Pb (3.52E-06)(1.05E-06)和gt; Ni (1.31E-06)(3.94E-07)的变化趋势为成人高于儿童。成人值(0.0002)大于儿童值(7.10E-05)。发现癌变风险平均值比允许限值高两倍(1 × 10−6)。
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来源期刊
Journal of Atmospheric Chemistry
Journal of Atmospheric Chemistry 地学-环境科学
CiteScore
4.60
自引率
5.00%
发文量
16
审稿时长
7.5 months
期刊介绍: The Journal of Atmospheric Chemistry is devoted to the study of the chemistry of the Earth''s atmosphere, the emphasis being laid on the region below about 100 km. The strongly interdisciplinary nature of atmospheric chemistry means that it embraces a great variety of sciences, but the journal concentrates on the following topics: Observational, interpretative and modelling studies of the composition of air and precipitation and the physiochemical processes in the Earth''s atmosphere, excluding air pollution problems of local importance only. The role of the atmosphere in biogeochemical cycles; the chemical interaction of the oceans, land surface and biosphere with the atmosphere. Laboratory studies of the mechanics in homogeneous and heterogeneous transformation processes in the atmosphere. Descriptions of major advances in instrumentation developed for the measurement of atmospheric composition and chemical properties.
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