Ferroelectrically Switchable Half-Quantized Hall Effect

IF 9.1 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY Nano Letters Pub Date : 2025-04-24 DOI:10.1021/acs.nanolett.5c00550
M. U. Muzaffar, Kai-Zhi Bai, Wei Qin, Guohua Cao, Bo Fu, Ping Cui, Shun-Qing Shen, Zhenyu Zhang
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Abstract

Integrating ferroelectricity, antiferromagnetism, and topological quantum transport within a single material is rare but crucial for developing next-generation quantum devices. Here, we propose a multiferroic heterostructure consisting of an antiferromagnetic MnBi2Te4 bilayer and an Sb2Te3 film is able to harbor the half-quantized Hall (HQH) effect with a ferroelectrically switchable Hall conductivity of ± e2/2h. We first show that, in the energetically stable configuration, the antiferromagnetic MnBi2Te4 bilayer opens a gap in the top surface bands of Sb2Te3 through the proximity effect, while its bottom surface bands remain gapless; consequently, an HQH conductivity of e2/2h can be sustained clockwise or counterclockwise, depending on the antiferromagnetic configuration of the MnBi2Te4. Remarkably, when interlayer sliding is applied within the MnBi2Te4 bilayer, its electric polarization direction associated with parity-time reversal symmetry breaking is reversed, accompanied by a reversal of the HQH conductivity. The proposed approach offers a powerful route to control topological quantum transport in antiferromagnetic materials by ferroelectricity.

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铁电可切换半量子化霍尔效应
在单一材料中集成铁电性、反铁磁性和拓扑量子输运是罕见的,但对于开发下一代量子器件至关重要。在这里,我们提出了一种由反铁磁MnBi2Te4双分子层和Sb2Te3薄膜组成的多铁异质结构,该异质结构能够具有半量子化霍尔(HQH)效应,其铁电可切换霍尔电导率为±e2/2h。我们首先表明,在能量稳定构型下,反铁磁性MnBi2Te4双分子层通过邻近效应在Sb2Te3的上表面带中打开了一个间隙,而其下表面带则保持无间隙;因此,根据MnBi2Te4的反铁磁结构,可以顺时针或逆时针维持e2/2h的HQH电导率。值得注意的是,当在MnBi2Te4双分子层内施加层间滑动时,其与奇偶时间反转对称性破缺相关的电极化方向被逆转,并伴随着HQH电导率的反转。该方法为利用铁电控制反铁磁材料中的拓扑量子输运提供了一条强有力的途径。
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来源期刊
Nano Letters
Nano Letters 工程技术-材料科学:综合
CiteScore
16.80
自引率
2.80%
发文量
1182
审稿时长
1.4 months
期刊介绍: Nano Letters serves as a dynamic platform for promptly disseminating original results in fundamental, applied, and emerging research across all facets of nanoscience and nanotechnology. A pivotal criterion for inclusion within Nano Letters is the convergence of at least two different areas or disciplines, ensuring a rich interdisciplinary scope. The journal is dedicated to fostering exploration in diverse areas, including: - Experimental and theoretical findings on physical, chemical, and biological phenomena at the nanoscale - Synthesis, characterization, and processing of organic, inorganic, polymer, and hybrid nanomaterials through physical, chemical, and biological methodologies - Modeling and simulation of synthetic, assembly, and interaction processes - Realization of integrated nanostructures and nano-engineered devices exhibiting advanced performance - Applications of nanoscale materials in living and environmental systems Nano Letters is committed to advancing and showcasing groundbreaking research that intersects various domains, fostering innovation and collaboration in the ever-evolving field of nanoscience and nanotechnology.
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