Effect of an ultrathin rare-earth Dy interlayer on the spin-orbit torques and interfacial Dyzaloshinskii-Moriya interaction in perpendicularly magnetized Pt/Dy/Co multilayers

IF 6.3 2区 材料科学 Q2 CHEMISTRY, PHYSICAL Journal of Alloys and Compounds Pub Date : 2025-05-10 Epub Date: 2025-04-24 DOI:10.1016/j.jallcom.2025.180607
Dong Li , Minrui Li , Yanping Lai , Xiyue Liu , Jijun Yun , Zhiyong Quan , Xiaohong Xu
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Abstract

Spin-source/ferromagnet interfaces in spin–orbit torque (SOT) devices play a significant role in efficient spin-current generation, transport and interfacial interactions. In this study, an ultrathin rare-earth Dy layer with a thickness of 0.6 nm was inserted into the Pt/Co interface to explore its impact on SOT-driven magnetization reversal. Anomalous Hall effect measurements reveal an increase of the damping-like SOT efficiency by ∼480 %, alongside a reduced switching current density of ∼6.68 × 106 A/cm2 in a perpendicularly magnetized Pt/Dy/Co/Ta stack. In particular, a notable increase of the field-like SOT efficiency by ∼1000 % and the large effective spin Hall angle of ∼0.491 reveal the enhanced interfacial Rashba spin–orbit coupling and/or spin transparency by the Dy decoration. More importantly, a field-free SOT reversal was observed, which may originate from the out-of-plane Rashba effective magnetic field owing to the lateral inhomogeneous component distribution between Dy and Co. Furthermore, an enhanced interfacial Dyzaloshinskii-Moriya interaction (DMI) was achieved in the Pt/Dy/Co/Ta stack. Our results demonstrate that interface engineering with an ultrathin rare-earth Dy interlayer can significantly strengthen the interfacial effects, such as interfacial spin–orbit coupling, spin transparency, and DMI, providing a promising approach to manufacturing energy-efficient SOT-based spin memories and racetrack devices.

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超薄稀土Dy中间层对垂直磁化Pt/Dy/Co多层膜自旋-轨道转矩和界面Dyzaloshinskii-Moriya相互作用的影响
自旋轨道力矩(SOT)器件中的自旋源/铁磁体界面在有效的自旋电流产生、传输和界面相互作用方面发挥着重要作用。本研究在铂/钴界面中插入了厚度为 0.6 纳米的超薄稀土镝层,以探索其对 SOT 驱动的磁化反转的影响。反常霍尔效应测量结果表明,在垂直磁化的 Pt/Dy/Co/Ta 堆栈中,阻尼样 SOT 效率提高了约 480%,开关电流密度降低了约 6.68×106 A/cm2。特别是,场样 SOT 效率显著提高了约 1000%,有效自旋霍尔角达到约 0.491,这表明镝装饰增强了界面 Rashba 自旋轨道耦合和/或自旋透明度。更重要的是,观察到了无场 SOT 反转,这可能源于 Dy 和 Co 之间横向不均匀分量分布所产生的面外 Rashba 有效磁场。此外,在铂/镝/钴/钽堆栈中还实现了增强的界面 Dyzaloshinskii-Moriya 相互作用(DMI)。我们的研究结果表明,使用超薄稀土镝中间膜的界面工程可以显著增强界面效应,如界面自旋轨道耦合、自旋透明度和 DMI,为制造基于 SOT 的高能效自旋存储器和赛道器件提供了一种可行的方法。
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来源期刊
Journal of Alloys and Compounds
Journal of Alloys and Compounds 工程技术-材料科学:综合
CiteScore
11.10
自引率
14.50%
发文量
5146
审稿时长
67 days
期刊介绍: The Journal of Alloys and Compounds is intended to serve as an international medium for the publication of work on solid materials comprising compounds as well as alloys. Its great strength lies in the diversity of discipline which it encompasses, drawing together results from materials science, solid-state chemistry and physics.
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