Evaluation of changes in buffer properties from an in-situ engineered barrier experiment

IF 5.3 2区 地球科学 Q2 CHEMISTRY, PHYSICAL Applied Clay Science Pub Date : 2023-08-08 DOI:10.1016/j.clay.2023.107092
Minseop Kim , Geon Young Kim , Jin-seop Kim , Seok Yoon , Changsoo Lee , DeukHwan Lee , Gi Jun Lee , Mihye Kong , Eun-soo Hong
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Abstract

The In-situ Demonstration of Engineering Barrier System (In-DEBS), a field test in Korea, commenced operations in July 2016 to showcase the complex thermal-hydraulic-mechanical behavior of the engineering barrier in a high-level radioactive waste repository. To emulate the actual repository, the In-DEBS test utilized a heater and buffer material comprised of compacted bentonite blocks. From January to October 2022, the In-DEBS buffer was sequentially dismantled, and the buffer samples were collected and analyzed for physical properties such as dry density and water content based on the sample location. The findings indicated that the physical properties of the In-DEBS buffer material showed variations, which may have been caused by various factors such as technical gaps, the dismantling process, and temperature gradient caused by heaters. This study also presents several experiments conducted on the samples obtained from the In-DEBS field test and compared with laboratory experimental data of untreated samples. The thermal conductivity and the hydraulic conductivity of the field-collected samples were lower than those of the untreated samples and the swelling properties of the samples were found to be influenced by their respective locations within the buffer, Although the empirical correlation based on laboratory data on untreated samples demonstrated high accuracy, some discrepancies were observed between the properties of field samples and the predicted values, highlighting the importance of field tests.

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从原位工程屏障实验中评估缓冲性能的变化
工程屏障系统的现场演示(in - debs)于2016年7月在韩国开始进行现场测试,以展示高放射性废物处置库中工程屏障的复杂热-水力-机械行为。为了模拟实际的储存库,In-DEBS测试使用了由压实膨润土块组成的加热器和缓冲材料。2022年1月至10月,依次拆除In-DEBS缓冲层,收集缓冲层样品,并根据样品位置分析干密度和含水量等物理性质。研究结果表明,In-DEBS缓冲材料的物理性能出现了变化,这可能是由技术差距、拆卸过程和加热器引起的温度梯度等多种因素引起的。本研究还介绍了对In-DEBS现场试验获得的样品进行的几项实验,并与未处理样品的实验室实验数据进行了比较。现场采集样品的热导率和水力导率低于未经处理的样品,并且发现样品的膨胀特性受到其在缓冲区内各自位置的影响。尽管基于未经处理样品的实验室数据的经验相关性显示出较高的准确性,但观察到现场样品的特性与预测值之间存在一些差异。强调实地试验的重要性。
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来源期刊
Applied Clay Science
Applied Clay Science 地学-矿物学
CiteScore
10.30
自引率
10.70%
发文量
289
审稿时长
39 days
期刊介绍: Applied Clay Science aims to be an international journal attracting high quality scientific papers on clays and clay minerals, including research papers, reviews, and technical notes. The journal covers typical subjects of Fundamental and Applied Clay Science such as: • Synthesis and purification • Structural, crystallographic and mineralogical properties of clays and clay minerals • Thermal properties of clays and clay minerals • Physico-chemical properties including i) surface and interface properties; ii) thermodynamic properties; iii) mechanical properties • Interaction with water, with polar and apolar molecules • Colloidal properties and rheology • Adsorption, Intercalation, Ionic exchange • Genesis and deposits of clay minerals • Geology and geochemistry of clays • Modification of clays and clay minerals properties by thermal and physical treatments • Modification by chemical treatments with organic and inorganic molecules(organoclays, pillared clays) • Modification by biological microorganisms. etc...
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