A step beyond in steady-state and time-resolved electro-optical spectroscopy: Demonstration of a customized simple, compact, low-cost, fiber-based interferometer system.

IF 2.3 2区 物理与天体物理 Q3 CHEMISTRY, PHYSICAL Structural Dynamics-Us Pub Date : 2022-01-13 eCollection Date: 2022-01-01 DOI:10.1063/4.0000134
Giovanni Pica, Daniele Bajoni, Giulia Grancini
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引用次数: 3

Abstract

Electro-optical spectroscopy is nowadays a routine approach for the analysis of light induced properties and dynamical processes in matter, whose understanding is particularly crucial for the intelligent design of novel synthetic materials and the engineering and optimization of high-impact optoelectronic devices. Currently, within this field, it is the common choice to rely on multiple commercial setups, often costly and complex, which can rarely combine multiple functions at the same time with the required sensitivity, resolution, and spectral tunability (in both excitation and detection). Here, we present an innovative, compact, and low-cost system based on "three in one" components for the simultaneous electro-optical material and device characterization. It relies on compact fiber-coupled Fourier transform spectroscopy, the core of the system, enabling a fast spectral analysis to acquire simultaneously wavelength and time resolved photoluminescence (PL) maps (as a function of the time and wavelength), PL quantum yield, and electroluminescence signal. Our system bypasses conventional ones, proposing a new solution for a compact, low-cost, and user-friendly tool, while maintaining high levels of resolution and sensitivity.

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在稳态和时间分辨电光光谱学上更进一步:一个定制的简单、紧凑、低成本、基于光纤的干涉仪系统的演示。
电光光谱学是当今分析物质光致特性和动力学过程的常规方法,对新型合成材料的智能设计和高冲击光电器件的工程设计和优化尤为重要。目前,在该领域,通常选择依赖多种商业设置,通常昂贵且复杂,很少能够同时结合所需的灵敏度,分辨率和光谱可调性(在激发和检测中)的多种功能。在这里,我们提出了一种基于“三合一”组件的创新,紧凑和低成本的系统,用于同时表征电光材料和器件。它依赖于紧凑的光纤耦合傅立叶变换光谱,该系统的核心,使快速光谱分析能够同时获得波长和时间分辨的光致发光(PL)图(作为时间和波长的函数),PL量子产率和电致发光信号。我们的系统绕过传统的,提出了一个新的解决方案,一个紧凑的,低成本的,用户友好的工具,同时保持高水平的分辨率和灵敏度。
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来源期刊
Structural Dynamics-Us
Structural Dynamics-Us CHEMISTRY, PHYSICALPHYSICS, ATOMIC, MOLECU-PHYSICS, ATOMIC, MOLECULAR & CHEMICAL
CiteScore
5.50
自引率
3.60%
发文量
24
审稿时长
16 weeks
期刊介绍: Structural Dynamics focuses on the recent developments in experimental and theoretical methods and techniques that allow a visualization of the electronic and geometric structural changes in real time of chemical, biological, and condensed-matter systems. The community of scientists and engineers working on structural dynamics in such diverse systems often use similar instrumentation and methods. The journal welcomes articles dealing with fundamental problems of electronic and structural dynamics that are tackled by new methods, such as: Time-resolved X-ray and electron diffraction and scattering, Coherent diffractive imaging, Time-resolved X-ray spectroscopies (absorption, emission, resonant inelastic scattering, etc.), Time-resolved electron energy loss spectroscopy (EELS) and electron microscopy, Time-resolved photoelectron spectroscopies (UPS, XPS, ARPES, etc.), Multidimensional spectroscopies in the infrared, the visible and the ultraviolet, Nonlinear spectroscopies in the VUV, the soft and the hard X-ray domains, Theory and computational methods and algorithms for the analysis and description of structuraldynamics and their associated experimental signals. These new methods are enabled by new instrumentation, such as: X-ray free electron lasers, which provide flux, coherence, and time resolution, New sources of ultrashort electron pulses, New sources of ultrashort vacuum ultraviolet (VUV) to hard X-ray pulses, such as high-harmonic generation (HHG) sources or plasma-based sources, New sources of ultrashort infrared and terahertz (THz) radiation, New detectors for X-rays and electrons, New sample handling and delivery schemes, New computational capabilities.
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Laser-induced electron diffraction: Imaging of a single gas-phase molecular structure with one of its own electrons. Deconvolution of dynamic heterogeneity in protein structure. Role of crystal orientation in attosecond photoinjection dynamics of germanium. CrysFormer: Protein structure determination via Patterson maps, deep learning, and partial structure attention. Introduction to the Special Issue Tribute to Olga Kennard (1924-2023).
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