First Measurements of Carbonaceous Aerosol across Urban, Rural and Residential Areas in Jeddah City, Saudi Arabia

IF 16.4 1区 化学 Q1 CHEMISTRY, MULTIDISCIPLINARY Accounts of Chemical Research Pub Date : 2021-06-01 DOI:10.5572/ajae.2021.021
Iqbal M. Ismail, Ahmad S. Summan, Jalal M. Basahi, Essam Hammam, Mohamed F. Yassin, Ibrahim A. Hassan
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Abstract

Concentrations of black carbon (BC), organic carbon (OC), and total suspended particulate matter (TSP) were simultaneously assessed in urban, rural and residential areas in Jeddah city for one year from January to December 2017. It was aimed in the present study to provide information about the spatial and seasonal variability of these aerosol species in Jeddah, and insight into sources, processes and effects of meteorological conditions. To the best of our knowledge, this is the first study investigating the variability of carbonaceous aerosols (OC and BC) in Saudi Arabia. The average concentrations of OC, BC, and TSP varied spatially and temporally. The annual average concentrations of OC, BC, and TSP were 134.05, 7.16, and 569.41 μg m−3 and 34.32, 5.14, and 240.64 μg m−3 and 10.67, 4.39 and 101.31 μg m−3 in the urban, residential and rural areas, respectively. Moreover, there was a clear seasonal variation in the concentration of carbonaceous aerosols; the highest concentrations were recorded in February and September, while the lowest concentrations of OC were recorded during April, May and August in the urban, residential and rural sites, respectively. Nevertheless, the lowest concentrations of BC were recorded during March in the urban and residential sites and during November in the rural site. The relative concentrations of OC and BC to the TSP were relatively high, and they have a significant correlation with prevalent wind speed (−0.636, and −0.581 in the urban area), (−0.539 and −0.511 in the residential area), and (−0.508 and −0.501 in the rural area), respectively. The marked differences in the concentrations of BC and OC were reflected on OC/BC ratio, which is a good representative of different source types. This preliminary study showed that the potential local sources were emissions from traffic (fossil fuel), biomass burning, anthropogenic activities (e.g. car drifting and outdoor cooking), and industrial activities. The present study suggest the presence of highly inefficient combustion sources and highlight the need for the regulation of such emissions.

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沙特阿拉伯吉达市城市、农村和居民区碳气溶胶的首次测量
2017年1月至12月,对吉达市城市、农村和居民区的黑碳(BC)、有机碳(OC)和总悬浮颗粒物(TSP)浓度进行了为期一年的监测。本研究的目的是提供吉达这些气溶胶种类的空间和季节变化信息,并深入了解气象条件的来源、过程和影响。据我们所知,这是第一个在沙特阿拉伯调查碳质气溶胶(OC和BC)变异性的研究。OC、BC和TSP的平均浓度存在时空差异。城市、居民和农村地区OC、BC和TSP的年平均浓度分别为134.05、7.16和569.41 μ m, 34.32、5.14和240.64 μ m, 10.67、4.39和101.31 μ m。此外,含碳气溶胶的浓度有明显的季节变化;城区、居民点和农村OC浓度分别在2月和9月最高,4月、5月和8月最低。然而,BC的最低浓度出现在3月份的城市和居民点,11月份的农村居民点。OC和BC相对于TSP的相对浓度较高,且与流行风速呈显著相关(城区为-0.636、-0.581),居民区为-0.539、-0.511,农村为-0.508、-0.501)。BC和OC浓度的显著差异体现在OC/BC比值上,OC/BC比值很好地代表了不同的源类型。这项初步研究表明,潜在的本地污染源包括交通(化石燃料)、生物质燃烧、人为活动(如汽车漂移和户外烹饪)和工业活动的排放。目前的研究表明,低效燃烧源的存在,并强调需要调节
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来源期刊
Accounts of Chemical Research
Accounts of Chemical Research 化学-化学综合
CiteScore
31.40
自引率
1.10%
发文量
312
审稿时长
2 months
期刊介绍: Accounts of Chemical Research presents short, concise and critical articles offering easy-to-read overviews of basic research and applications in all areas of chemistry and biochemistry. These short reviews focus on research from the author’s own laboratory and are designed to teach the reader about a research project. In addition, Accounts of Chemical Research publishes commentaries that give an informed opinion on a current research problem. Special Issues online are devoted to a single topic of unusual activity and significance. Accounts of Chemical Research replaces the traditional article abstract with an article "Conspectus." These entries synopsize the research affording the reader a closer look at the content and significance of an article. Through this provision of a more detailed description of the article contents, the Conspectus enhances the article's discoverability by search engines and the exposure for the research.
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