Legion: An Instrument for High-Throughput Electrochemistry

IF 4.6 Q1 CHEMISTRY, ANALYTICAL ACS Measurement Science Au Pub Date : 2023-07-13 DOI:10.1021/acsmeasuresciau.3c00022
Benjamin H. R. Gerroll, Krista M. Kulesa, Charles A. Ault and Lane A. Baker*, 
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引用次数: 1

Abstract

Electrochemical arrays promise utility for accelerated hypothesis testing and breakthrough discoveries. Herein, we report a new high-throughput electrochemistry platform, colloquially called “Legion,” for applications in electroanalysis and electrosynthesis. Legion consists of 96 electrochemical cells dimensioned to match common 96-well plates that are independently controlled with a field-programmable gate array. We demonstrate the utility of Legion by measuring model electrochemical probes, pH-dependent electron transfers, and electrocatalytic dehalogenation reactions. We consider advantages and disadvantages of this new instrumentation, with the hope of expanding the electrochemical toolbox.

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军团:高通量电化学仪器
电化学阵列有望加速假设检验和突破性发现。在此,我们报告了一种新的高通量电化学平台,俗称“军团”,用于电分析和电合成。Legion由96个电化学电池组成,尺寸与普通的96孔板相匹配,这些板由现场可编程门阵列独立控制。我们通过测量模型电化学探针、ph依赖的电子转移和电催化脱卤反应来证明Legion的实用性。我们考虑了这种新仪器的优点和缺点,希望扩大电化学工具箱。
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来源期刊
ACS Measurement Science Au
ACS Measurement Science Au 化学计量学-
CiteScore
5.20
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0.00%
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0
期刊介绍: ACS Measurement Science Au is an open access journal that publishes experimental computational or theoretical research in all areas of chemical measurement science. Short letters comprehensive articles reviews and perspectives are welcome on topics that report on any phase of analytical operations including sampling measurement and data analysis. This includes:Chemical Reactions and SelectivityChemometrics and Data ProcessingElectrochemistryElemental and Molecular CharacterizationImagingInstrumentationMass SpectrometryMicroscale and Nanoscale systemsOmics (Genomics Proteomics Metabonomics Metabolomics and Bioinformatics)Sensors and Sensing (Biosensors Chemical Sensors Gas Sensors Intracellular Sensors Single-Molecule Sensors Cell Chips Arrays Microfluidic Devices)SeparationsSpectroscopySurface analysisPapers dealing with established methods need to offer a significantly improved original application of the method.
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