Numerical investigations on hydrothermal flame characteristics of water-cooled hydrothermal burner

IF 1.6 4区 工程技术 Q3 Chemical Engineering International Journal of Chemical Reactor Engineering Pub Date : 2023-07-11 DOI:10.1515/ijcre-2023-0040
Yiran Geng, Shuzhong Wang, Fan Zhang, Zicheng Li, Xinyin Zhang, Yanhui Li, Wenqiang He
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Abstract

Abstract Supercritical hydrothermal combustion, as a quick homogeneous oxidizing process, offers a promising treatment option for industrial wastewater. This paper established a computational fluid dynamics model of a water-cooled hydrothermal combustion burner to investigate the thermal flame characteristics. The effects of the fuel mass flow rate, fuel concentration, initial reactor temperature, reaction pressure, and oxidant temperature on the thermal combustion ignition were revealed. The results indicate that the fuel concentration (from 10 wt% to 60 wt%) and initial reactor temperature (from 623 to 773 K) had less effect on the ignition temperature. In contrast, the ignition temperature increases by 398 K with increasing fuel mass flow rate (from 24 kg h−1 to 1080 kg h−1). As the oxygen temperature increases (from 273 to 673 K), the ignition temperature gradually decreases to 573 K and then increases. An increase in reaction pressure can facilitate a decrease in ignition temperature to a certain extent, and the optimal reaction pressure is 25 MPa. This study provides a vital reference for a hydrothermal burner’s scale-up design and ignition operation.
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水冷式水热燃烧器水热火焰特性的数值研究
摘要超临界水热燃烧作为一种快速均相氧化工艺,为工业废水的处理提供了一种很有前途的选择。本文建立了水冷式水热燃烧器的计算流体动力学模型,对其热火焰特性进行了研究。揭示了燃料质量流量、燃料浓度、反应器初始温度、反应压力和氧化剂温度对热燃烧点火的影响。结果表明,燃油浓度(从10 wt%至60 wt%)和初始反应器温度(从623到773 K) 对点火温度的影响较小。相反,点火温度增加398 K随燃油质量流量的增加(从24 公斤 h−1至1080 公斤 h−1)。随着氧气温度的升高(从273升至673 K) ,点火温度逐渐降低至573 K,然后增加。反应压力的增加可以在一定程度上促进点火温度的降低,最佳反应压力为25 MPa。该研究为水热燃烧器的放大设计和点火操作提供了重要参考。
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来源期刊
CiteScore
2.80
自引率
12.50%
发文量
107
审稿时长
3 months
期刊介绍: The International Journal of Chemical Reactor Engineering covers the broad fields of theoretical and applied reactor engineering. The IJCRE covers topics drawn from the substantial areas of overlap between catalysis, reaction and reactor engineering. The journal is presently edited by Hugo de Lasa and Charles Xu, counting with an impressive list of Editorial Board leading specialists in chemical reactor engineering. Authors include notable international professors and R&D industry leaders.
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