Experimental and analytical investigation on resin impregnation behavior in continuous carbon fiber reinforced thermoplastic polyimide composites

Shota Kazano, Toshiko Osada, Satoshi Kobayashi, Ken Goto
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引用次数: 10

Abstract

In molding of carbon fiber reinforced thermoplastics (CFRTP), resin impregnation behavior to fiber yarns is very important because higher viscosity of molten thermoplastics inhibites resin impregnation to the interspace among fibers. Resultant resin un-impregnation causes lower mechanical properties of CFRTP. The purpose of this study was to clarify the relation among molding method, molding conditions and resin impregnation to fiber yarns experimentally and analytically. In this study, CFRTPs using continuous carbon fiber yarn as a reinforcement and a thermoplastic polyimide which is excellent in heat resistance as a matrix resin were produced by Micro-Braiding, Film Stacking and Powder method. In addition resin impregnation was modeled based on Darcy’s law and continuity condition. As a result, analytical resin impregnation prediction showed good agreements with the experimental results in all the producing methods and molding conditions. In addition, the void content in the molded CFRP could be greatly reduced by pressurizing cooling.

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连续碳纤维增强热塑性聚酰亚胺复合材料树脂浸渍性能的实验与分析研究
在碳纤维增强热塑性塑料(CFRTP)的成型中,树脂对纤维纱线的浸渍行为是非常重要的,因为熔融热塑性塑料的高粘度抑制了树脂对纤维间隙的浸渍。树脂未浸渍导致CFRTP的力学性能降低。通过实验和分析,阐明了成型方法、成型条件和树脂浸渍对纤维纱线的影响。本研究以连续碳纤维纱为增强材料,以耐热性能优良的热塑性聚酰亚胺为基体树脂,采用微编织法、叠膜法和粉末法制备了CFRTPs。基于达西定律和连续性条件对树脂浸渍过程进行了建模。结果表明,在各种生产方法和成型条件下,树脂浸渍分析预测结果与实验结果吻合较好。此外,加压冷却可以大大降低CFRP成型中的空隙含量。
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