3D Printing Technology for Short-continuous Carbon Fiber Synchronous Reinforced Thermoplastic Composites: A Comparison between Towpreg Extrusion and In Situ Impregnation Processes

Fuji Wang , Gongshuo Wang , Hongquan Wang , Rao Fu , Yajing Lei , Jianing He
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Abstract

Three-dimensional (3D) printing of carbon fiber-reinforced thermoplastic composites (CFRTPs) provides an effective method for manufacturing the CFRTPs parts with complex structures. To increase the mechanical performance of these parts, a 3D printing technology for short-continuous carbon fiber synchronous-reinforced thermoplastic composites (S/C-CFRTPs) has been proposed. However, the synchronous reinforcement that existed only at particular positions led to a limited improvement in the mechanical performance of the 3D-printed S/C-CFRTP part, which made it challenging to meet the engineering requirements. To solve this problem, two methods for achieving synchronous reinforcement at all the positions of the 3D-printed S/C-CFRTP part are proposed. To determine a suitable printing process for the S/C-CFRTP part, a comprehensive comparison between the two methods was conducted through theoretical analysis and experimental verification, involving the printing mechanism, fiber content, impregnation percentage, and mechanical performance. The results indicated that the towpreg extrusion process was suitable for manufacturing the 3D-printed S/C-CFRTP part. Compared with the in situ impregnation process, the towpreg extrusion process led to a fiber content increase of approximately 7% and void rate reduction of approximately 6%, resulting in 19% and 20% increases in the tensile and flexural strengths of the 3D-printed S/C-CFRTPs, respectively. Additionally, an optimized process parameter setting for fabricating an S/C-CFRTP prepreg filament with excellent mechanical performance was proposed. The findings of this study can provide a new approach for further improving the mechanical performance of the 3D-printed advanced composites.

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短连续碳纤维同步增强热塑性复合材料的3D打印技术——Towpreg挤出和原位浸渍工艺的比较
碳纤维增强热塑性复合材料(CFRTP)的三维(3D)打印为制造具有复杂结构的CFRTP零件提供了一种有效的方法。为了提高这些零件的力学性能,提出了一种短连续碳纤维同步增强热塑性复合材料(S/C-CFRTP)的3D打印技术。然而,仅存在于特定位置的同步补强导致3D打印S/C-CFRTP零件的机械性能得到有限的改善,这使得满足工程要求具有挑战性。为了解决这个问题,提出了两种在3D打印S/C-CFRTP零件的所有位置实现同步加固的方法。为了确定S/C-CFRTP零件的合适印刷工艺,通过理论分析和实验验证,对两种方法进行了全面的比较,包括印刷机理、纤维含量、浸渍率和机械性能。结果表明,丝束预浸料挤出工艺适用于制造3D打印S/C-CFRTP零件。与原位浸渍工艺相比,丝束预浸料挤出工艺使纤维含量增加了约7%,空隙率降低了约6%,使3D打印的S/C-CFRTP的拉伸和弯曲强度分别提高了19%和20%。此外,还提出了制备具有优异机械性能的S/C-CFRTP预浸料长丝的优化工艺参数设置。这项研究的发现可以为进一步提高3D打印先进复合材料的力学性能提供一种新的方法。
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