Structural evolution from disordered to fibrous assembly via a dual visual dissipative pathway†

IF 6 2区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY Materials Chemistry Frontiers Pub Date : 2023-09-05 DOI:10.1039/D3QM00864A
Kui Wang, Xin Meng and Xue-Jiao Zhang
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Abstract

In this work, calixpyridinium was found to be a good building block for constructing an unusual artificial dissipative system with a proton donor by using an alkali as the fuel. Inspired by this, the structural evolution from disordered to fibrous assembly based on a calixpyridinium–indigo carmine system via a dual visual dissipative pathway with an alkali as the fuel was achieved. This was further applied in mimicking an alkaline biological molecule-driven dissipative process in real samples.

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通过双重视觉耗散途径从无序组装到纤维组装的结构演变†
在这项工作中,杯吡啶被发现是一个很好的构建块,可以通过使用碱作为燃料构建一个具有质子供体的不寻常的人工耗散系统。受此启发,以碱为燃料,通过双视觉耗散途径,实现了基于联吡啶-靛蓝胭脂红体系的从无序到纤维组装的结构演变。这进一步应用于模拟真实样品中碱性生物分子驱动的耗散过程。
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来源期刊
Materials Chemistry Frontiers
Materials Chemistry Frontiers Materials Science-Materials Chemistry
CiteScore
12.00
自引率
2.90%
发文量
313
期刊介绍: Materials Chemistry Frontiers focuses on the synthesis and chemistry of exciting new materials, and the development of improved fabrication techniques. Characterisation and fundamental studies that are of broad appeal are also welcome. This is the ideal home for studies of a significant nature that further the development of organic, inorganic, composite and nano-materials.
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