APPLICABILITY OF BRAY-LIEBHAFSKY REACTION FOR CHEMICAL COMPUTING

Ž. Čupić, Ana I vanović Šašić, S. Maćešić, S. Anic, Ljiljana Kolar- Anić
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Abstract

The first discovered homogeneous oscillatory reaction was the Bray-Liebhafsky (BL) one, described in a paper published exactly 100 years ago. However, the applicability of oscillatory reactions in chemical computing was recently discovered. Here we intend to expose the native computing concept applied to intermittent states of the BL reaction, because we believe that this particular state may have some advantages. For this purpose, numerical simulations will be used based on the known model. Sequences of perturbations will be introduced by adding iodate (IO3-) and hydrogen peroxide (H2O2), separately, as well as in various combinations with one another. It will be shown that dynamic states obtained after perturbations with same species depend very much on the sequence in which these species were used in perturbations. Additionally, it will be shown that obtained dynamic states shift the system from chaotic intermittent dynamic state to different complex periodic states. Hence, the applicability of the BL reaction system in chemical computing was demonstrated.
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bray-liebhafsky反应在化学计算中的适用性
第一个发现的均相振荡反应是布雷-利勃哈夫斯基反应(BL),该反应在整整100年前发表的一篇论文中有描述。然而,振荡反应在化学计算中的适用性最近才被发现。在这里,我们打算将原生计算概念应用于BL反应的间歇状态,因为我们相信这种特定的状态可能有一些优势。为此,将在已知模型的基础上进行数值模拟。通过分别添加碘酸盐(IO3-)和过氧化氢(H2O2),以及以各种组合方式引入扰动序列。将会证明,在相同物种的扰动后得到的动态状态在很大程度上取决于在扰动中使用这些物种的顺序。此外,所获得的动态状态将使系统从混沌的间歇动态状态转变为不同的复杂周期状态。从而证明了BL反应体系在化学计算中的适用性。
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