Room temperature operation of InAs quantum dot lasers formed by diblock-copolymer lithography and selective area MOCVD growth

Honghyuk Kim, Wei Wei, T. Kuech, P. Gopalan, L. Mawst
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引用次数: 2

Abstract

Semiconductor Laser diodes (LD) employing quantum dot (QD) active regions have attracted attention due to the theoretical predictions: low threshold current density and low temperature sensitivity originated from the delta-function-like density of states and small active volume [1]. However, while high performance devices have been demonstrated, the realization of all the predicted advantages has remained challenging. Self-assembled QDs grown by Stranski-Krastanov (SK) growth mode can suffer from an inhomogeneity in the QD size distribution, as well as an inherent wetting layer [2]. Nanopatterning and selective metalorganic chemical vapor deposition (MOCVD) growth offer a more controllable pathway for QD formation, allowing the QD size to be decoupled from the strain state of the material. This process results in the formation of dense arrays of wetting-layer-free QDs, although the challenges stemming from surface state formation and efficient carrier injection into the QDs remain problematic issues [3]. As such, previously reported LDs employing these In0.3Ga0.7As QD active regions only operate at low temperatures [3]. It has been contended that embedding the SK QDs within an InGaAs quantum well (QW) improves carrier capture into the quantum dots [4]. Here, we demonstrate an In0.1Ga0.9As QW placed adjacent to a wetting layer-free InAs QD active region leads to improved active region carrier collection, allowing for room temperature (RT) lasing. The LDs employ an active region consisting of a dense single-layer array of compressively-strained InAs QDs (Density ∼ 4×1010cm−2), selectively grown by MOCVD on top of a 4nm thick In0.1Ga0.9As QW.
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双嵌段共聚物光刻和选择性MOCVD生长形成的InAs量子点激光器的室温操作
采用量子点(QD)有源区的半导体激光二极管(LD)因其具有低阈值电流密度和低温度灵敏度(源于类似于δ函数的态密度)和小有源体积([1])的理论预测而备受关注。然而,虽然高性能器件已经被证明,但实现所有预测的优势仍然具有挑战性。采用Stranski-Krastanov (SK)生长方式生长的自组装量子点在尺寸分布上存在不均匀性,并且存在固有的湿润层[2]。纳米图和选择性金属有机化学气相沉积(MOCVD)生长为量子点形成提供了更可控的途径,允许量子点尺寸与材料的应变状态解耦。这一过程形成了致密的无润湿层量子点阵列,尽管来自表面态形成和有效载流子注入量子点的挑战仍然是有待解决的问题。因此,先前报道的采用这些In0.3Ga0.7As量子点有源区域的ld只能在低温下工作。有人认为,将SK量子点嵌入InGaAs量子阱(QW)可以改善量子点[4]的载流子捕获。在这里,我们展示了放置在无润湿层InAs量子点有源区域附近的In0.1Ga0.9As量子点w,可以改善有源区域载流子收集,从而实现室温(RT)激光。该ld采用由密集的单层压缩应变InAs量子点阵列(密度~ 4×1010cm−2)组成的有源区域,通过MOCVD选择性地生长在4nm厚的In0.1Ga0.9As量子点上。
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