Research on the electrical characteristics of atmospheric strong ionization dielectric barrier discharge for air pollution control

Prince Junior Asilevi, Daniel Akambawe, Chengwu Yu, Jue Li, Patrick Boakye, Sampson Oduro-Kwarteng, Muhammad Imran Nawaz
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Abstract

The specific input energy (SIE), current density, and discharge power of homemade strong ionization dielectric barrier discharge (DBD) were studied to suppress gas-phase benzene at atmospheric pressure efficiently. Findings indicate that for 300 ppm of benzene at 3.5 kJ/L SIE, benzene's removal efficiency reached 96%. The decline in current density by 66.48% and 43.7% for an initial benzene concentration of 300 ppm was due to increased oxygen content (from 2.4% to 20.9%) and relative humidity (from 18.9% to 90%), respectively, thus reducing electron concentration and consequentially enhanced the removal efficiency over 93%.Furthermore, the decomposition law's beta parameter decreased from 3.1 kJ/L at 300 ppm to 1.6 kJ/L at 100 ppm, indicating that •O and •OH radicals are key species for the decomposition of benzene and electron dissociation reactions largely control the process. The Maxwell– Boltzmann electron energy distribution function was solved using the average energy of the strong ionization discharge reactor (~10 eV), showing that approximately 84.8 % of high energy electrons possess enough energy to cause the benzene ring cleavage and free radical production. The study results show that the strong ionization DBD plasma reactor is highly efficient in removing benzene from industrial waste air, hence air pollution control.
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大气强电离介质阻挡放电的电学特性研究
研究了自制强电离介质阻挡放电(DBD)在常压下抑制气相苯的比输入能量(SIE)、电流密度和放电功率。结果表明,当苯浓度为300 ppm、SIE为3.5 kJ/L时,苯的去除率可达96%。当苯的初始浓度为300 ppm时,由于氧含量(从2.4%增加到20.9%)和相对湿度(从18.9%增加到90%)的增加,电流密度分别下降了66.48%和43.7%,从而降低了电子浓度,从而使去除率提高了93%以上。此外,分解规律的β参数从300 ppm时的3.1 kJ/L下降到100 ppm时的1.6 kJ/L,说明•O和•OH自由基是苯分解的关键基团,电子解离反应在很大程度上控制了苯的分解过程。利用强电离放电反应器(~10 eV)的平均能量求解麦克斯韦-玻尔兹曼电子能量分布函数,表明约84.8%的高能电子具有足够的能量引起苯环裂解和自由基的产生。研究结果表明,强电离DBD等离子体反应器对工业废气中苯的去除效果良好,可有效控制大气污染。
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