Optical Properties of 1D ZnO/MoS\(_2\) Heterostructures Synthesized by Thermal Evaporation Method

Thi Thu Giang Luu, Q. Do, M. Tran, T. Nguyen, D. H. Nguyen, T. Pham
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Abstract

MoS2 material attracts a great attention from researchers due to its graphene-like structure and the bandgap difference between its hexagonal monolayer and bulks. Recently, ZnO/MoS2 heterostructures have been received significant interest due to their distinguished properties. In this study, one-dimensional ZnO and ZnO/MoS2 heterostructures were successfully synthesized by a thermal co-evaporation method. Compare with ZnO, the band-to-band emission of ZnO/MoS2 heterostructures establishes a “blueshift” towards a shorter wavelength. It could be explained by the lattice strain in ZnO/MoS2 heterostructures due to the difference of primitive cell of ZnO and MoS2. Additionally, the quench in the visible region of the PL spectrum of ZnO/MoS2 heterostructures also explains the reduction of the defect in ZnO due to the presence of MoS2.
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热蒸发法制备一维ZnO/MoS \(_2\)异质结构的光学性质
二硫化钼材料由于其类石墨烯结构以及其六方单层与块体之间的带隙差异而备受关注。近年来,氧化锌/二硫化钼异质结构因其独特的性能而受到广泛关注。在本研究中,通过热共蒸发方法成功合成了一维ZnO和ZnO/MoS2异质结构。与ZnO相比,ZnO/MoS2异质结构的波段间发射形成了向短波长的“蓝移”。这可以解释为ZnO/MoS2异质结构中的晶格应变,这是由于ZnO和MoS2的原始细胞不同造成的。此外,ZnO/MoS2异质结构的PL光谱可见区域的猝灭也解释了由于MoS2的存在而导致ZnO缺陷的减少。
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