From 232Th(n, n’γ) cross sections to level production and total neutron inelastic scattering cross sections

Nicolas Dari Bako, M. Kerveno, P. Dessagne, C. Borcea, M. Boromiza, R. Capote, François Claeys, M. Dupuis, G. Henning, A. Negret, M. Nyman, A. Olăcel, Eliot Party, A. Plompen
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Abstract

To probe the neutron inelastic scattering off 232Th, an experiment took place at the EC-JRC Geel conducted with the experimental setup GRAPhEME to detect emitted γ-rays. The prompt γ-ray spectroscopy method was used and 70 experimental 232Th(n, n’γ) cross sections were obtained from the experimental data. Combining these cross sections, nuclear-structure data available in databases and hypotheses to complete the latter, neutron inelastic level production cross sections in 232Th and the total inelastic cross section were calculated. For the first time, the total inelastic cross section of an actinide nucleus was derived on the total neutron energy range from experimental data only. Comparisons of (n, n’) cross section data with evaluated data reveal a good agreement between them all above 300 keV of neutron energy. TALYS calculations are compatible but lower than the evaluated data.
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从232Th(n, n′γ)截面到能级产生和总中子非弹性散射截面
为了探测232Th的中子非弹性散射,在EC-JRC Geel用实验装置GRAPhEME进行了一项实验,以探测发射的γ射线。采用提示γ射线能谱法,从实验数据中得到了70个实验232Th(n, n′γ)截面。结合这些截面、数据库中的核结构数据和假设来完成后者,计算了232Th中子非弹性能级产生截面和总非弹性截面。首次从实验数据出发,在中子总能量范围上推导了锕系原子核的总非弹性截面。(n, n’)截面数据与评价数据的比较表明,它们在300 keV以上的中子能量上符合得很好。TALYS的计算是兼容的,但低于评估的数据。
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