Lead isotopic ratios in European atmospheric aerosols

A. Bollhöfer, K.J.R. Rosman
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引用次数: 33

Abstract

Aerosols collected between 1994 and 1999 at more than 45 different sites in Europe have been measured for Pb isotopic composition and Pb concentrations by Thermal Ionisation Mass Spectrometry (TIMS). With respect to 206Pb/207Pb and 208Pb/207Pb ratios a change in isotopic composition compared with earlier measurements was detected in parts of Europe. Also, seasonal variations were observed at some sites. This was most probably due to a relative increase (due to the phasing out of leaded petrol) of both industrial Pb in the atmosphere and pollution from long- or meso-scale transport.

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欧洲大气气溶胶中的铅同位素比率
利用热电离质谱法(TIMS)测量了1994年至1999年间在欧洲超过45个不同地点收集的气溶胶的Pb同位素组成和Pb浓度。关于206Pb/207Pb和208Pb/207Pb比值,在欧洲部分地区发现了与早期测量相比的同位素组成变化。此外,在一些地点观察到季节变化。这很可能是由于大气中工业铅的相对增加(由于逐步淘汰含铅汽油)和来自长尺度或中尺度运输的污染。
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