Detailed spectroscopy in the superdeformed second minimum of 240 Pu

Abstract

Spectroscopic studies in the superdeformed shape isomer of 240Pu using γ-spectroscopy, conversion electron spectroscopy and transmission resonance spectroscopy have been performed. In a high-resolution and high-efficiency γ-spectroscopy experiment the out-of-band decays of several excited superdeformed rotational sequences with K=2− and 1− could be identified together with evidence for a weakly populated 0− octupole band. Surprisingly, no low-lying collective quadrupole excitations could be observed. Complementary information could be obtained in conversion electron measurements in coincidence with isomeric fission, resulting in the first identification of the lowest s-vibrational K=0+ band. For all rotational bands the variation of the moment of inertia with spin could be studied. A predominant population of negative parity states in the second well could be observed, which can be explained by the selective population and depopulation of the second minimum. Complementary transmission resonance measurements have been performed, yielding new information on the fine structure of high-lying (s-)vibrational multi-phonon states. A new method could be established to determine the excitation energy of the fission isomer ground state from measured level densities.