Solar-light-induced green conversion of amines into imines by lemon derived heteroatoms-doped GQDs as a green photocatalyst

IF 16.4 1区 化学 Q1 CHEMISTRY, MULTIDISCIPLINARY Accounts of Chemical Research Pub Date : 2022-12-23 DOI:10.3233/mgc-220094
Satyam Singh, R. Yadav, T. W. Kim, P. Pande, Surabhi Chaubey, Ashutosh Kumar Singh
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引用次数: 1

Abstract

Graphene is one of the amazing present encroachments in current research area of science and one of the utmost fascinating materials for relevance in cutting-edge research. Herein, we designed lemon-derived heteroatoms-doped graphene quantum dots (S, N-GQDs) based photocatalyst for the first time. For the integrating reactions of amines in aerobic conditions under solar light by S, N-GQDs photocatalyst exhibit utmost higher photocatalytic activity than simple oxygen-doped graphene quantum dots (O-GQDs) due to slow recombination charges. The mechanisms accountable for the drastically increased photocatalytic activity of S, N-GQDs in solar light responsive integrating reactions of amines in aerobic conditions into the corresponding derivative of imines are also completely scrutinized.
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柠檬衍生杂原子掺杂GQDs作为绿色光催化剂在日光诱导下将胺转化为亚胺
石墨烯是当前科学研究领域中令人惊叹的新进展之一,也是与前沿研究相关的最具吸引力的材料之一。本文首次设计了柠檬衍生的杂原子掺杂石墨烯量子点(S, N-GQDs)光催化剂。由于复合电荷缓慢,N-GQDs光催化剂表现出比单纯掺氧石墨烯量子点(O-GQDs)更高的光催化活性。S, N-GQDs在好氧条件下对太阳光响应的胺与相应亚胺衍生物的整合反应中的光催化活性急剧增加的机制也得到了全面的审查。
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来源期刊
Accounts of Chemical Research
Accounts of Chemical Research 化学-化学综合
CiteScore
31.40
自引率
1.10%
发文量
312
审稿时长
2 months
期刊介绍: Accounts of Chemical Research presents short, concise and critical articles offering easy-to-read overviews of basic research and applications in all areas of chemistry and biochemistry. These short reviews focus on research from the author’s own laboratory and are designed to teach the reader about a research project. In addition, Accounts of Chemical Research publishes commentaries that give an informed opinion on a current research problem. Special Issues online are devoted to a single topic of unusual activity and significance. Accounts of Chemical Research replaces the traditional article abstract with an article "Conspectus." These entries synopsize the research affording the reader a closer look at the content and significance of an article. Through this provision of a more detailed description of the article contents, the Conspectus enhances the article's discoverability by search engines and the exposure for the research.
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