Migration characteristics of oil pollutants into soil pores influenced by surface wettability

IF 3.6 4区 环境科学与生态学 Q2 BIOCHEMISTRY & MOLECULAR BIOLOGY Environmental Pollutants and Bioavailability Pub Date : 2022-09-28 DOI:10.1080/26395940.2022.2128885
Lingqi Lin, Yulin Pu, Di Wang, Xi Guo, Peng Wang, Zhong Lu
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Abstract

ABSTRACT Pore-scale modeling plays an indispensable role in unveiling the migration mechanism of oil pollutants into the water-saturated soil. Navier Stokes equations and conservation of mass, coupled with the phase field method, are employed to investigate the effect of soil wettability on oil pollutants migration into the soil porous media. The results show that the oil-water interface in the migration process does not advance evenly in three wetting states. When the model system is in oil-wetting state, oil pollutants obviously migrate at a higher speed. Through monitoring the evolution of oil front location and analyzing the velocity distribution vertical to the flow direction at the central axis of the model, the channel corresponding to the peak velocity is the dominant flow channel for the oil pollutants. This study will have the potential ability in obtaining the pore-scale migration regulation of oil pollutions as well as more accurately predicting the pollution range.
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表面润湿性对石油污染物向土壤孔隙迁移特性的影响
孔隙尺度模拟对于揭示含油污染物进入饱和水土壤的运移机理具有不可缺少的作用。采用Navier Stokes方程和质量守恒方程,结合相场法研究了土壤润湿性对石油污染物向土壤多孔介质迁移的影响。结果表明:在三种润湿状态下,运移过程中油水界面的推进并不均匀;当模型系统处于油润湿状态时,油类污染物运移速度明显加快。通过监测油锋位置的演变,分析模型中轴线处垂直于流向的流速分布,发现峰值流速所对应的通道是油污染物的主导流动通道。本研究将有可能获得油类污染在孔隙尺度上的运移规律,更准确地预测污染范围。
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来源期刊
Environmental Pollutants and Bioavailability
Environmental Pollutants and Bioavailability Chemical Engineering-Chemical Health and Safety
CiteScore
4.30
自引率
3.00%
发文量
47
审稿时长
13 weeks
期刊介绍: Environmental Pollutants & Bioavailability is a peer-reviewed open access forum for insights on the chemical aspects of pollutants in the environment and biota, and their impacts on the uptake of the substances by living organisms. Topics include the occurrence, distribution, transport, transformation, transfer, fate, and effects of environmental pollutants, as well as their impact on living organisms. Substances of interests include heavy metals, persistent organic pollutants, and emerging contaminants, such as engineered nanomaterials, as well as pharmaceuticals and personal-care products as pollutants.
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