Second Harmonic Generation in Periodical Metal-Insulator-Metal Nanoparticle Arrays

Sebastian Beer, Jeetendra Gour, Umair Mir, A. Alberucci, U. Zeitner, Stefan Nolte
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Abstract

The collective oscillation of free electrons in metals (plasmon) leads to a localized field enhancement at the surface. Structures with periodically arranged metallic nano-particles possess two plasmonic resonances: one from the individual nano-particles (localized surface plasmon resonance, LSPR) and one from the collective response triggered by the periodic arrangement (surface lattice resonance, SLR) [1]. Whereas the LSPR is fixed by the sample geometry, the spectral position of the SLR is tuneable with the optical angle of incidence. Both the resonances as well as plasmonic nano-gaps are associated to a strong field enhancement, which can boost nonlinear optical effects.
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周期性金属-绝缘体-金属纳米颗粒阵列的二次谐波产生
金属(等离子体)中自由电子的集体振荡导致表面局部场增强。金属纳米粒子周期性排列的结构具有两种等离子体共振:一种来自单个纳米粒子(局部表面等离子体共振,LSPR),另一种来自周期性排列引发的集体响应(表面晶格共振,SLR)[1]。单反的光谱位置随入射角度的变化而变化,而LSPR是由样品的几何形状决定的。共振和等离子体纳米间隙都与强场增强有关,这可以增强非线性光学效应。
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