Radon Progeny Recoil Effect in Retrospective Indoor Glass Dosimetry

C. D. Tibambre-Heredia, H. Olaya-Dávila, A. C. Sevilla, Rahul Samasundaram, Jorge López, S. Martinez-Ovalle, L. Sajo-Bohus
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Abstract

Radon gas diffusion and progeny transport in air, are mechanisms to be considered in retrospective glass dosimetry.   With the aim to contribute to the understanding of the Rn progeny recoil energy role in this dosimetry methodology, we carried out a simulation employing GEANT4 code. In that, we assumed the chemical compound of the glass that is used commonly in households.  Results are compared to experimentally measured 210Bi concentration to show that the recoil energy helps the progenies incrustation, mainly for the 218,214Po alpha emitters but do not influence bismuth-210 diffusion directly. A significant difference exists between our results and measured values; that is interpreted as due to atomic displacement by primary knock-on atoms. The SiO2 molecule binding energy breaks and the following ion recombination, induce a structural modification between the atom by e.g. cavities formation in such a way that reduces significantly the radon progeny diffusion speed.
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回顾性室内玻璃剂量测定中的氡子代反冲效应
氡气体在空气中的扩散和子代输运是回顾性玻璃剂量法中要考虑的机制。为了更好地理解Rn子代反冲能量在该剂量学方法中的作用,我们使用GEANT4代码进行了模拟。在这里,我们假设了家庭中常用的玻璃的化合物。结果与实验测量的210Bi浓度进行了比较,结果表明反冲能量对铋-210的扩散没有直接影响,主要对218,214Po α发射体有促进作用。我们的结果与测量值之间存在显著差异;这被解释为原子位移是由初级撞击原子引起的。SiO2分子结合能的断裂和随后的离子复合,导致原子之间的结构改变,例如形成空腔,从而显著降低氡子体的扩散速度。
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