Source apportionment and source-specific risk evaluation of potential toxic elements in oasis agricultural soils of Tarim River Basin.

IF 3.9 2区 综合性期刊 Q1 MULTIDISCIPLINARY SCIENCES Scientific Reports Pub Date : 2023-02-20 DOI:10.1038/s41598-023-29911-3
Yizhen Li, Jilili Abuduwaili, Long Ma, Wen Liu, Tao Zeng
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Abstract

As rapidly developing area of intensive agriculture during the past half century, the oases in the source region of the Tarim River have encountered serious environmental challenges. Therefore, a comparative analysis of soil pollution characteristics and source-specific risks in different oases is an important measure to prevent and control soil pollution and provide guidance for extensive resource management in this area. In this study, the concentration of potential toxic elements (PTEs) was analyzed by collecting soil samples from the four oases in the source region of the Tarim River. The cumulative frequency curve method, pollution index method, positive matrix factorization (PMF) model, geographical detector method and health risk assessment model were used to analyze the pollution status and source-specific risk of potential toxic elements in different oases. The results showed that Cd was the most prominent PTE in the oasis agricultural soil in the source region of the Tarim River. Especially in Hotan Oasis, where 81.25% of the soil samples were moderately contaminated and 18.75% were highly contaminated with Cd. The PTEs in the Hotan Oasis corresponded to a moderate level of risk to the ecological environment, and the noncarcinogenic risk of soil PTEs in the four oases to local children exceeded the threshold (TH > 1), while the carcinogenic risk to local residents was acceptable (1E-06 < TCR < 1E-04). The research results suggested that the Hotan Oasis should be the key area for soil pollution control in the source region of the Tarim River, and agricultural activities and natural sources, industrial sources, and atmospheric dust fall are the priority sources that should be controlled in the Aksu Oasis, Kashgar Oasis and Yarkant River Oasis, respectively. The results of this study provide important decision-making support for the protection and management of regional agricultural soil and the environment.

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塔里木河流域绿洲农业土壤潜在有毒元素源解析及源特异性风险评价
塔里木河源区绿洲作为近半个世纪以来集约化农业快速发展的地区,面临着严峻的环境挑战。因此,比较分析不同绿洲土壤污染特征和源性风险是防治土壤污染和指导该地区资源粗放管理的重要措施。本研究通过采集塔里木河源区4个绿洲土壤样品,分析了土壤中潜在有毒元素(PTEs)的浓度。采用累积频率曲线法、污染指数法、正矩阵分解(PMF)模型、地理探测器法和健康风险评价模型对不同绿洲的污染状况和潜在有毒元素的源特异性风险进行了分析。结果表明,Cd是塔里木河源区绿洲农业土壤中最显著的PTE。特别是和田绿洲,81.25%的土壤样本Cd中度污染,18.75%的土壤样本Cd高度污染。和田绿洲土壤pte对生态环境的风险水平为中等,4个绿洲土壤pte对当地儿童的非致癌风险均超过阈值(TH > 1),对当地居民的致癌风险为可接受的(1E-06)
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来源期刊
Scientific Reports
Scientific Reports Natural Science Disciplines-
CiteScore
7.50
自引率
4.30%
发文量
19567
审稿时长
3.9 months
期刊介绍: We publish original research from all areas of the natural sciences, psychology, medicine and engineering. You can learn more about what we publish by browsing our specific scientific subject areas below or explore Scientific Reports by browsing all articles and collections. Scientific Reports has a 2-year impact factor: 4.380 (2021), and is the 6th most-cited journal in the world, with more than 540,000 citations in 2020 (Clarivate Analytics, 2021). •Engineering Engineering covers all aspects of engineering, technology, and applied science. It plays a crucial role in the development of technologies to address some of the world''s biggest challenges, helping to save lives and improve the way we live. •Physical sciences Physical sciences are those academic disciplines that aim to uncover the underlying laws of nature — often written in the language of mathematics. It is a collective term for areas of study including astronomy, chemistry, materials science and physics. •Earth and environmental sciences Earth and environmental sciences cover all aspects of Earth and planetary science and broadly encompass solid Earth processes, surface and atmospheric dynamics, Earth system history, climate and climate change, marine and freshwater systems, and ecology. It also considers the interactions between humans and these systems. •Biological sciences Biological sciences encompass all the divisions of natural sciences examining various aspects of vital processes. The concept includes anatomy, physiology, cell biology, biochemistry and biophysics, and covers all organisms from microorganisms, animals to plants. •Health sciences The health sciences study health, disease and healthcare. This field of study aims to develop knowledge, interventions and technology for use in healthcare to improve the treatment of patients.
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