封闭环境中长期原位空气质量评价:气相色谱离子迁移谱适用性研究。

IF 1.1 4区 化学 Q4 PHYSICS, ATOMIC, MOLECULAR & CHEMICAL European Journal of Mass Spectrometry Pub Date : 2023-08-01 DOI:10.1177/14690667231187502
Pedro Catalão Moura, Valentina Vassilenko
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引用次数: 1

摘要

现代人的生活大多是在室内空间度过的,比如私人住宅、工作场所、车辆和公共设施。然而,这些封闭环境中的空气质量往往很差,导致人们接触到大量有毒和有害化合物。挥发性有机化合物(VOCs)是造成封闭空间空气质量差的主要因素之一,此外,其中一些对人体有机体特别有害。考虑到这一事实,我们在室内使用气相色谱-离子迁移谱(GC-IMS)设备进行了1年多的每日现场空气分析。结果表明,10种挥发性有机化合物全年都存在于室内空气中,对控制空气质量尤为重要。这些化合物分别是乙酸、丙酮、苯、丁醇、乙醇、异丁醇、丙酸、丙醇、2-丙醇和叔丁基甲基醚。研究了分析期内总挥发性有机化合物(tVOCs)强度的变化规律及连续月份间的相对变化规律。观察到,tVOCs的总体趋势与全年气温的变化密切相关,表明两者具有较强的相关性。从这项研究中获得的结果证明了数据的高质量和相关性,突出了气相色谱- ims在室内环境中长期现场空气质量评估的适用性,从而确定了在短期和长期接触情况下对人体机体的潜在健康风险。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

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Long-term in situ air quality assessment in closed environments: A gas chromatography-ion mobility spectrometry applicability study.

Contemporary life is mostly spent in indoor spaces like private houses, workplaces, vehicles and public facilities. Nonetheless, the air quality in these closed environments is often poor which leads to people being exposed to a vast range of toxic and hazardous compounds. Volatile organic compounds (VOCs) are among the main factors responsible for the lack of air quality in closed spaces and, in addition, some of them are particularly hazardous to the human organism. Considering this fact, we conducted daily in situ air analyses over 1 year using a gas chromatography-ion mobility spectrometry (GC-IMS) device in an indoor location. The obtained results show that 10 VOCs were consistently present in the indoor air throughout the entire year, making them particularly important for controlling air quality. All of these compounds were successfully identified, namely acetic acid, acetone, benzene, butanol, ethanol, isobutanol, propanoic acid, propanol, 2-propanol and tert-butyl methyl ether. The behaviour of the total VOCs (tVOCs) intensity during the period of analysis and the relative variation between consecutive months were studied. It was observed that the overall trend of tVOCs closely mirrored the variation of air temperature throughout the year suggesting their strong correlation. The results obtained from this study demonstrate the high quality and relevance of the data, highlighting the suitability of GC-IMS for in situ long-term air quality assessment in indoor environments and, consequently, for identifying potential health risks for the human organism in both short-term and long-term exposure scenarios.

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来源期刊
CiteScore
2.40
自引率
7.70%
发文量
16
审稿时长
>12 weeks
期刊介绍: JMS - European Journal of Mass Spectrometry, is a peer-reviewed journal, devoted to the publication of innovative research in mass spectrometry. Articles in the journal come from proteomics, metabolomics, petroleomics and other areas developing under the umbrella of the “omic revolution”.
期刊最新文献
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